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@ARTICLE{Hildenbrand:910837,
author = {Hildenbrand, Felix and Aupperle, Felix and Stahl, Gereon
and Figgmeier, Egbert and Sauer, Dirk Uwe},
title = {{S}election of {E}lectrolyte {A}dditive {Q}uantities for
{L}ithium‐{I}on {B}atteries {U}sing {B}ayesian
{O}ptimization},
journal = {Batteries $\&$ supercaps},
volume = {5},
number = {7},
issn = {2566-6223},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2022-04187},
pages = {e202200038},
year = {2022},
abstract = {The composition of the liquid electrolyte is a key factor
inlifetime performance of lithium-ion batteries. The
selection andquantification of additives to the electrolyte
is an active field ofresearch. This study focuses on finding
the optimal additivecombination of fluoroethylene carbonate
(FEC) and vinylenecarbonate (VC) for NMC622-Graphite cells.
The central goal ofthis work is to accelerate the
experimental search in a largesearch area by using a
Bayesian-optimization algorithm toguide the search.
Different measurements are used as targetvariable such as
open-circuit voltage gradient and coulombicefficiency.
Consequentially, the capability of these measurementsfor
accelerated lifetime prediction compared to
conventionalageing tests by cycling is investigated. The
searchgathered and confirmed additive combinations with
excellentperformance after four iterations with a total of
15 additivecombinations analyzed. The results of this study
give insightsinto the interaction of VC and FEC with regard
to ageing.},
cin = {IEK-12 / JARA-ENERGY},
ddc = {620},
cid = {I:(DE-Juel1)IEK-12-20141217 / $I:(DE-82)080011_20140620$},
pnm = {1223 - Batteries in Application (POF4-122)},
pid = {G:(DE-HGF)POF4-1223},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000774000900001},
doi = {10.1002/batt.202200038},
url = {https://juser.fz-juelich.de/record/910837},
}