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@ARTICLE{MartinezCastro:910866,
author = {Martinez-Castro, Jose and Bolat, Rustem and Fan, Qitang and
Werner, Simon and Arefi, Hadi H. and Esat, Taner and
Sundermeyer, Jörg and Wagner, Christian and Michael
Gottfried, J. and Temirov, Ruslan and Ternes, Markus and
Stefan Tautz, F.},
title = {{D}isentangling the electronic structure of an adsorbed
graphene nanoring by scanning tunneling microscopy},
journal = {Communications materials},
volume = {3},
number = {1},
issn = {2662-4443},
address = {London},
publisher = {Springer Nature},
reportid = {FZJ-2022-04216},
pages = {57},
year = {2022},
abstract = {Graphene nanorings are promising model structures to
realize persistent ring currents and Aharonov–Bohm effect
at the single molecular level. To investigate such
intriguing effects, precise molecular characterization is
crucial. Here, we combine low-temperature scanning tunneling
imaging and spectroscopy with CO functionalized tips and
algorithmic data analysis to investigate the electronic
structure of the molecular cycloarene C108 (graphene
nanoring) adsorbed on a Au(111) surface. We demonstrate that
CO functionalized tips enhance the visibility of molecular
resonances, both in differential conductance spectra and in
real-space topographic images. Comparing our experimental
data with ab-initio density functional theory reveals a
remarkably precise agreement of the molecular orbitals and
enables us to disentangle close-lying molecular states only
separated by 50 meV at an energy of 2 eV below the Fermi
level. We propose this combination of techniques as a
promising new route for a precise electronic
characterization of complex molecules and other physical
properties which have electronic resonances in the
tip-sample junction.},
cin = {PGI-3 / JARA-FIT},
ddc = {600},
cid = {I:(DE-Juel1)PGI-3-20110106 / $I:(DE-82)080009_20140620$},
pnm = {5213 - Quantum Nanoscience (POF4-521)},
pid = {G:(DE-HGF)POF4-5213},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000844772400001},
doi = {10.1038/s43246-022-00275-x},
url = {https://juser.fz-juelich.de/record/910866},
}