000911136 001__ 911136
000911136 005__ 20240712084621.0
000911136 0247_ $$2doi$$a10.1111/jace.18678
000911136 0247_ $$2ISSN$$a0002-7820
000911136 0247_ $$2ISSN$$a1551-2916
000911136 0247_ $$2Handle$$a2128/32452
000911136 0247_ $$2WOS$$aWOS:000832787300001
000911136 037__ $$aFZJ-2022-04452
000911136 082__ $$a660
000911136 1001_ $$aLu, Kimbal T.$$b0
000911136 245__ $$aLnUO4‐based glass–ceramic composites as waste forms for the immobilization of lanthanide‐bearing uranium wastes
000911136 260__ $$aWesterville, Ohio$$bSoc.$$c2022
000911136 3367_ $$2DRIVER$$aarticle
000911136 3367_ $$2DataCite$$aOutput Types/Journal article
000911136 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1667900808_13125
000911136 3367_ $$2BibTeX$$aARTICLE
000911136 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000911136 3367_ $$00$$2EndNote$$aJournal Article
000911136 520__ $$aWe report a comprehensive study on lanthanide monouranate–based glass–ceramic (GC) composites as potential waste forms for the immobilization of the lanthanide actinide fraction waste arising from the reprocessing of spent nuclear fuel (SNF). Although the crystalline LnUO4 precursor prepared via a nitrate route can be well stabilized in a sodium aluminoborosilicate glass, the in situ crystallization of EuUO4 in glass from oxide precursors (Eu2O3 and U3O8) is rather robust with regards to various processing conditions such as waste loadings, ceramic-to-glass ratios, and cooling rates. Scanning electron microscopy and transmission electron microscopy investigations revealed the detailed microstructures, where ∼1–5-μm spheres for NdUO4 and EuUO4, and ∼1–5-μm rectangular crystals for DyUO4 and HoUO4 were observed in residual glasses. As designed, the pentavalent uranium has been confirmed by diffuse reflectance spectroscopy. Overall, LnUO4-based GC composite waste forms are chemically durable, offering flexible processing options with wide operating windows for SNF and process waste stream management.
000911136 536__ $$0G:(DE-HGF)POF4-1411$$a1411 - Nuclear Waste Disposal (POF4-141)$$cPOF4-141$$fPOF IV$$x0
000911136 588__ $$aDataset connected to CrossRef, Journals: juser.fz-juelich.de
000911136 7001_ $$00000-0001-6321-4696$$aZhang, Yingjie$$b1$$eCorresponding author
000911136 7001_ $$0P:(DE-HGF)0$$aWei, Tao$$b2
000911136 7001_ $$0P:(DE-Juel1)176900$$aMurphy, Gabriel$$b3$$ufzj
000911136 7001_ $$0P:(DE-HGF)0$$aBhuiyan, Aurpa$$b4
000911136 7001_ $$0P:(DE-HGF)0$$aScales, Nicholas$$b5
000911136 7001_ $$0P:(DE-HGF)0$$aZheng, Rongkun$$b6
000911136 773__ $$0PERI:(DE-600)2008170-4$$a10.1111/jace.18678$$gVol. 105, no. 12, p. 7697 - 7709$$n12$$p7697 - 7709$$tJournal of the American Ceramic Society$$v105$$x0002-7820$$y2022
000911136 8564_ $$uhttps://juser.fz-juelich.de/record/911136/files/Journal%20of%20the%20American%20Ceramic%20Society%20-%202022%20-%20Lu%20-%20LnUO4%E2%80%90based%20glass%20ceramic%20composites%20as%20waste%20forms%20for%20the.pdf$$yOpenAccess
000911136 909CO $$ooai:juser.fz-juelich.de:911136$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000911136 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)176900$$aForschungszentrum Jülich$$b3$$kFZJ
000911136 9131_ $$0G:(DE-HGF)POF4-141$$1G:(DE-HGF)POF4-140$$2G:(DE-HGF)POF4-100$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF4-1411$$aDE-HGF$$bForschungsbereich Energie$$lNukleare Entsorgung, Sicherheit und Strahlenforschung (NUSAFE II)$$vNukleare Entsorgung$$x0
000911136 9141_ $$y2022
000911136 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2021-01-27
000911136 915__ $$0LIC:(DE-HGF)CCBYNCND4$$2HGFVOC$$aCreative Commons Attribution-NonCommercial-NoDerivs CC BY-NC-ND 4.0
000911136 915__ $$0StatID:(DE-HGF)3001$$2StatID$$aDEAL Wiley$$d2021-01-27$$wger
000911136 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2021-01-27
000911136 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000911136 915__ $$0StatID:(DE-HGF)0420$$2StatID$$aNationallizenz$$d2022-11-22$$wger
000911136 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2022-11-22
000911136 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2022-11-22
000911136 915__ $$0StatID:(DE-HGF)1160$$2StatID$$aDBCoverage$$bCurrent Contents - Engineering, Computing and Technology$$d2022-11-22
000911136 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2022-11-22
000911136 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2022-11-22
000911136 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bJ AM CERAM SOC : 2021$$d2022-11-22
000911136 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2022-11-22
000911136 915__ $$0StatID:(DE-HGF)0600$$2StatID$$aDBCoverage$$bEbsco Academic Search$$d2022-11-22
000911136 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bASC$$d2022-11-22
000911136 915__ $$0StatID:(DE-HGF)9900$$2StatID$$aIF < 5$$d2022-11-22
000911136 9201_ $$0I:(DE-Juel1)IEK-6-20101013$$kIEK-6$$lNukleare Entsorgung$$x0
000911136 9801_ $$aFullTexts
000911136 980__ $$ajournal
000911136 980__ $$aVDB
000911136 980__ $$aUNRESTRICTED
000911136 980__ $$aI:(DE-Juel1)IEK-6-20101013
000911136 981__ $$aI:(DE-Juel1)IFN-2-20101013