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000911204 1001_ $$0P:(DE-HGF)0$$aWang, Lina$$b0
000911204 245__ $$aStrain Modulation for Light‐Stable n–i–p Perovskite/Silicon Tandem Solar Cells
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000911204 520__ $$aPerovskite/silicon tandem solar cells are promising to penetrate photovoltaicmarket. However, the wide-bandgap perovskite absorbers used in top-celloften suffer severe phase segregation under illumination, which restricts theoperation lifetime of tandem solar cells. Here, a strain modulation strategyto fabricate light-stable perovskite/silicon tandem solar cells is reported. Byemploying adenosine triphosphate, the residual tensile strain in the wide-bandgapperovskite absorber is successfully converted to compressive strain,which mitigates light-induced ion migration and phase segregation. Basedon the wide-bandgap perovskite with compressive strain, single-junctionsolar cells with the n–i–p layout yield a power conversion efficiency (PCE) of20.53% with the smallest voltage deficits of 440 mV. These cells also maintain83.60% of initial PCE after 2500 h operation at the maximum power point.Finally, these top cells are integrated with silicon bottom cells in a monolithictandem device, which achieves a PCE of 26.95% and improved light stabilityat open-circuit.
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000911204 536__ $$0G:(BMWi)0324275E$$aVerbundvorhaben: Street - Einsatz von hocheffizienten Solarzellen in elektrisch betriebenen Nutzfahrzeugen; Teilvorhaben: Herstellung und Entwicklung von (0324275E)$$c0324275E$$x1
000911204 536__ $$0G:(BMWi)0324351$$aTouch - Technologie- und Charakterisierungsplattform für die Entwicklung von hoch-effizienten Silizium-Heterostruktursolarzellen (0324351)$$c0324351$$x2
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000911204 7001_ $$0P:(DE-HGF)0$$aSong, Qizhen$$b1
000911204 7001_ $$0P:(DE-HGF)0$$aPei, Fengtao$$b2
000911204 7001_ $$0P:(DE-HGF)0$$aChen, Yihua$$b3$$eCorresponding author
000911204 7001_ $$0P:(DE-HGF)0$$aDou, Jie$$b4
000911204 7001_ $$0P:(DE-HGF)0$$aWang, Hao$$b5
000911204 7001_ $$0P:(DE-HGF)0$$aShi, Congbo$$b6
000911204 7001_ $$0P:(DE-HGF)0$$aZhang, Xiao$$b7
000911204 7001_ $$0P:(DE-HGF)0$$aFan, Rundong$$b8
000911204 7001_ $$0P:(DE-HGF)0$$aZhou, Wentao$$b9
000911204 7001_ $$0P:(DE-HGF)0$$aQiu, Zhiwen$$b10
000911204 7001_ $$0P:(DE-HGF)0$$aKang, Jiaqian$$b11
000911204 7001_ $$0P:(DE-HGF)0$$aWang, Xueyun$$b12
000911204 7001_ $$0P:(DE-Juel1)130263$$aLambertz, Andreas$$b13$$ufzj
000911204 7001_ $$0P:(DE-HGF)0$$aSun, Mengru$$b14
000911204 7001_ $$0P:(DE-HGF)0$$aNiu, Xiuxiu$$b15
000911204 7001_ $$0P:(DE-HGF)0$$aMa, Yue$$b16
000911204 7001_ $$0P:(DE-HGF)0$$aZhu, Cheng$$b17
000911204 7001_ $$0P:(DE-HGF)0$$aZhou, Huanping$$b18
000911204 7001_ $$0P:(DE-HGF)0$$aHong, Jiawang$$b19
000911204 7001_ $$0P:(DE-HGF)0$$aBai, Yang$$b20
000911204 7001_ $$0P:(DE-Juel1)169946$$aDuan, Weiyuan$$b21$$eCorresponding author$$ufzj
000911204 7001_ $$0P:(DE-Juel1)130233$$aDing, Kaining$$b22$$ufzj
000911204 7001_ $$0P:(DE-HGF)0$$aChen, Qi$$b23$$eCorresponding author
000911204 773__ $$0PERI:(DE-600)1474949-X$$a10.1002/adma.202201315$$gVol. 34, no. 26, p. 2201315 -$$n26$$p2201315 -$$tAdvanced materials$$v34$$x0935-9648$$y2022
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