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000911424 1001_ $$0P:(DE-HGF)0$$aRath, Purna Chandra$$b0
000911424 245__ $$aTape-cast Ce-substituted Li 7 La 3 Zr 2 O 12 electrolyte for improving electrochemical performance of solid-state lithium batteries
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000911424 520__ $$aSolid-state lithium-metal batteries (SSLMBs) with a composite solid electrolyte (CSE) have great potential forachieving both high energy density and high safety and are thus promising next-generation energy storagedevices. The current bottlenecks are a high electrode/electrolyte interface resistance and the limited Li+conductivity of the solid electrolyte layer. To reduce the interface resistance, a tape casting method isused to directly deposit a CSE layer (20 mm) onto a model LiFePO4 cathode. The CSE slurry infiltratesthe cathode layer, forming a Li+ conduction network and ensuring intimate contact between the CSEand the cathode. The tape casting parameters, such as the polymer/Li salt ratio, inorganic filler fraction,and casting thickness, for the CSE layer are investigated. To increase Li+ conductivity, Ce substitution isconducted for Li7 La3Zr2−xCexO 12, x ¼ 0–0.15. The effects of Ce content on the specific capacity, ratecapability, and cycling stability of Li//CSE//LiFePO4 cells are systematically studied. Li 7 La3Zr1.9 Ce0.1O 12(i.e., x ¼ 0.1) is found to be the optimal composition; it outperforms Li7 La3Zr2O 12 andLi 6.25Ga0.25 La3Zr2O12 in terms of CSE conductivity and SSLMB charge–discharge performance.
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000911424 7001_ $$0P:(DE-HGF)0$$aJheng, Yu-Syuan$$b1
000911424 7001_ $$0P:(DE-HGF)0$$aChen, Cheng-Chia$$b2
000911424 7001_ $$0P:(DE-Juel1)156244$$aTsai, Chih-Long$$b3
000911424 7001_ $$00000-0002-5989-1317$$aSu, Yu-Sheng$$b4
000911424 7001_ $$00000-0002-3832-9800$$aYang, Chun-Chen$$b5
000911424 7001_ $$0P:(DE-Juel1)156123$$aEichel, Rüdiger-A.$$b6
000911424 7001_ $$00000-0002-1053-8635$$aHsieh, Chien-Te$$b7
000911424 7001_ $$00000-0002-1695-1201$$aLee, Tai-Chou$$b8
000911424 7001_ $$00000-0002-8359-5817$$aChang, Jeng-Kuei$$b9$$eCorresponding author
000911424 773__ $$0PERI:(DE-600)2702232-8$$a10.1039/D2TA06808G$$gVol. 10, no. 42, p. 22512 - 22522$$n42$$p22512 - 22522$$tJournal of materials chemistry / A$$v10$$x2050-7488$$y2022
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