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@ARTICLE{Rath:911424,
      author       = {Rath, Purna Chandra and Jheng, Yu-Syuan and Chen,
                      Cheng-Chia and Tsai, Chih-Long and Su, Yu-Sheng and Yang,
                      Chun-Chen and Eichel, Rüdiger-A. and Hsieh, Chien-Te and
                      Lee, Tai-Chou and Chang, Jeng-Kuei},
      title        = {{T}ape-cast {C}e-substituted {L}i 7 {L}a 3 {Z}r 2 {O} 12
                      electrolyte for improving electrochemical performance of
                      solid-state lithium batteries},
      journal      = {Journal of materials chemistry / A},
      volume       = {10},
      number       = {42},
      issn         = {2050-7488},
      address      = {London ˜[u.a.]œ},
      publisher    = {RSC},
      reportid     = {FZJ-2022-04707},
      pages        = {22512 - 22522},
      year         = {2022},
      abstract     = {Solid-state lithium-metal batteries (SSLMBs) with a
                      composite solid electrolyte (CSE) have great potential
                      forachieving both high energy density and high safety and
                      are thus promising next-generation energy storagedevices.
                      The current bottlenecks are a high electrode/electrolyte
                      interface resistance and the limited Li+conductivity of the
                      solid electrolyte layer. To reduce the interface resistance,
                      a tape casting method isused to directly deposit a CSE layer
                      (20 mm) onto a model LiFePO4 cathode. The CSE slurry
                      infiltratesthe cathode layer, forming a Li+ conduction
                      network and ensuring intimate contact between the CSEand the
                      cathode. The tape casting parameters, such as the polymer/Li
                      salt ratio, inorganic filler fraction,and casting thickness,
                      for the CSE layer are investigated. To increase Li+
                      conductivity, Ce substitution isconducted for Li7
                      La3Zr2−xCexO 12, x ¼ 0–0.15. The effects of Ce content
                      on the specific capacity, ratecapability, and cycling
                      stability of Li//CSE//LiFePO4 cells are systematically
                      studied. Li 7 La3Zr1.9 Ce0.1O 12(i.e., x ¼ 0.1) is found to
                      be the optimal composition; it outperforms Li7 La3Zr2O 12
                      andLi 6.25Ga0.25 La3Zr2O12 in terms of CSE conductivity and
                      SSLMB charge–discharge performance.},
      cin          = {IEK-9},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {1223 - Batteries in Application (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1223},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000870375800001},
      doi          = {10.1039/D2TA06808G},
      url          = {https://juser.fz-juelich.de/record/911424},
}