Hauptseite > Publikationsdatenbank > Tape-cast Ce-substituted Li 7 La 3 Zr 2 O 12 electrolyte for improving electrochemical performance of solid-state lithium batteries > print

001     911424
005     20240712112813.0
024 7 _ |a 10.1039/D2TA06808G
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024 7 _ |a 2050-7488
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024 7 _ |a 2050-7496
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024 7 _ |a 2128/32906
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024 7 _ |a WOS:000870375800001
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037 _ _ |a FZJ-2022-04707
082 _ _ |a 530
100 1 _ |a Rath, Purna Chandra
|0 P:(DE-HGF)0
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245 _ _ |a Tape-cast Ce-substituted Li 7 La 3 Zr 2 O 12 electrolyte for improving electrochemical performance of solid-state lithium batteries
260 _ _ |a London ˜[u.a.]œ
|c 2022
|b RSC
336 7 _ |a article
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520 _ _ |a Solid-state lithium-metal batteries (SSLMBs) with a composite solid electrolyte (CSE) have great potential forachieving both high energy density and high safety and are thus promising next-generation energy storagedevices. The current bottlenecks are a high electrode/electrolyte interface resistance and the limited Li+conductivity of the solid electrolyte layer. To reduce the interface resistance, a tape casting method isused to directly deposit a CSE layer (20 mm) onto a model LiFePO4 cathode. The CSE slurry infiltratesthe cathode layer, forming a Li+ conduction network and ensuring intimate contact between the CSEand the cathode. The tape casting parameters, such as the polymer/Li salt ratio, inorganic filler fraction,and casting thickness, for the CSE layer are investigated. To increase Li+ conductivity, Ce substitution isconducted for Li7 La3Zr2−xCexO 12, x ¼ 0–0.15. The effects of Ce content on the specific capacity, ratecapability, and cycling stability of Li//CSE//LiFePO4 cells are systematically studied. Li 7 La3Zr1.9 Ce0.1O 12(i.e., x ¼ 0.1) is found to be the optimal composition; it outperforms Li7 La3Zr2O 12 andLi 6.25Ga0.25 La3Zr2O12 in terms of CSE conductivity and SSLMB charge–discharge performance.
536 _ _ |a 1223 - Batteries in Application (POF4-122)
|0 G:(DE-HGF)POF4-1223
|c POF4-122
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588 _ _ |a Dataset connected to CrossRef, Journals: juser.fz-juelich.de
700 1 _ |a Jheng, Yu-Syuan
|0 P:(DE-HGF)0
|b 1
700 1 _ |a Chen, Cheng-Chia
|0 P:(DE-HGF)0
|b 2
700 1 _ |a Tsai, Chih-Long
|0 P:(DE-Juel1)156244
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700 1 _ |a Su, Yu-Sheng
|0 0000-0002-5989-1317
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700 1 _ |a Yang, Chun-Chen
|0 0000-0002-3832-9800
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700 1 _ |a Eichel, Rüdiger-A.
|0 P:(DE-Juel1)156123
|b 6
700 1 _ |a Hsieh, Chien-Te
|0 0000-0002-1053-8635
|b 7
700 1 _ |a Lee, Tai-Chou
|0 0000-0002-1695-1201
|b 8
700 1 _ |a Chang, Jeng-Kuei
|0 0000-0002-8359-5817
|b 9
|e Corresponding author
773 _ _ |a 10.1039/D2TA06808G
|g Vol. 10, no. 42, p. 22512 - 22522
|0 PERI:(DE-600)2702232-8
|n 42
|p 22512 - 22522
|t Journal of materials chemistry / A
|v 10
|y 2022
|x 2050-7488
856 4 _ |y OpenAccess
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