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@INPROCEEDINGS{Park:911526,
      author       = {Park, Junbeom and Kretzschmar, Ansgar and Selmert, Victor
                      and Camara, Osmane and Kungl, Hans and Tempel, Hermann and
                      Basak, Shibabrata and Eichel, Rüdiger-A.},
      title        = {{UNDERSTANDING} {GAS} {ADSORPTION} {OF} {PAN}-{BASED}
                      {CARBON} {NANOFIBERS}},
      reportid     = {FZJ-2022-04786},
      year         = {2022},
      abstract     = {Polyacrylonitrile-based carbon nanofibers (PAN-based CNFs)
                      have great potential to be used for carbon dioxide (CO2)
                      capture due to their excellent CO2 adsorption properties.
                      The porous structure of PAN-based CNFs originates from their
                      turbostratic structure, which is composed of numerous
                      disordered stacks of graphitic layers. During the
                      carbonization process, the internal structure is arranged
                      toward the ordered graphitic structure, which significantly
                      influences the gas adsorption properties of PAN-based CNFs.
                      However, the relation between structural transformation and
                      CO2 capture is still not clear enough to tune the PAN-based
                      CNFs. In this paper, we show that, with increasing
                      carbonization temperature, the arrangement of the PAN-based
                      CNF’s structure along the stack and lateral directions
                      takes place independently: gradually aligning and merging
                      along the stack direction and enlarging along the lateral
                      direction. Further, we correlate the structural arrangement
                      and the CO2 adsorption properties of the PAN-based CNFs to
                      propose a comprehensive structural mechanism. This mechanism
                      provides the knowledge to understand and tailor the gas
                      adsorption properties of PAN-based CNFs.},
      month         = {May},
      date          = {2022-05-08},
      organization  = {PICO2022, Kasteel Vaalsbroek
                       (Netherlands), 8 May 2022 - 12 May
                       2022},
      subtyp        = {After Call},
      cin          = {IEK-9},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {1232 - Power-based Fuels and Chemicals (POF4-123) / iNEW2.0
                      (BMBF-03SF0627A) / Electroscopy - Electrochemistry of
                      All-solid-state-battery Processes using Operando Electron
                      Microscopy (892916) / HITEC - Helmholtz Interdisciplinary
                      Doctoral Training in Energy and Climate Research (HITEC)
                      (HITEC-20170406)},
      pid          = {G:(DE-HGF)POF4-1232 / G:(DE-Juel1)BMBF-03SF0627A /
                      G:(EU-Grant)892916 / G:(DE-Juel1)HITEC-20170406},
      typ          = {PUB:(DE-HGF)24},
      url          = {https://juser.fz-juelich.de/record/911526},
}