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000916492 005__ 20240712101018.0
000916492 0247_ $$2doi$$a10.1021/acs.est.1c07121
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000916492 0247_ $$2ISSN$$a1520-5851
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000916492 0247_ $$2pmid$$a35579536
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000916492 1001_ $$00000-0003-3462-2126$$aStockwell, Chelsea E.$$b0$$eCorresponding author
000916492 245__ $$aAirborne Emission Rate Measurements Validate Remote Sensing Observations and Emission Inventories of Western U.S. Wildfires
000916492 260__ $$aColumbus, Ohio$$bAmerican Chemical Society$$c2022
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000916492 520__ $$aCarbonaceous emissions from wildfires are a dynamic mixture of gases and particles that have important impacts on air quality and climate. Emissions that feed atmospheric models are estimated using burned area and fire radiative power (FRP) methods that rely on satellite products. These approaches show wide variability and have large uncertainties, and their accuracy is challenging to evaluate due to limited aircraft and ground measurements. Here, we present a novel method to estimate fire plume-integrated total carbon and speciated emission rates using a unique combination of lidar remote sensing aerosol extinction profiles and in situ measured carbon constituents. We show strong agreement between these aircraft-derived emission rates of total carbon and a detailed burned area-based inventory that distributes carbon emissions in time using Geostationary Operational Environmental Satellite FRP observations (Fuel2Fire inventory, slope = 1.33 ± 0.04, r2 = 0.93, and RMSE = 0.27). Other more commonly used inventories strongly correlate with aircraft-derived emissions but have wide-ranging over- and under-predictions. A strong correlation is found between carbon monoxide emissions estimated in situ with those derived from the TROPOspheric Monitoring Instrument (TROPOMI) for five wildfires with coincident sampling windows (slope = 0.99 ± 0.18; bias = 28.5%). Smoke emission coefficients (g MJ–1) enable direct estimations of primary gas and aerosol emissions from satellite FRP observations, and we derive these values for many compounds emitted by temperate forest fuels, including several previously unreported species.
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000916492 7001_ $$00000-0002-3998-9990$$aBela, Megan M.$$b1
000916492 7001_ $$00000-0002-5763-1925$$aCoggon, Matthew M.$$b2
000916492 7001_ $$0P:(DE-Juel1)184937$$aGkatzelis, Georgios$$b3$$ufzj
000916492 7001_ $$00000-0003-1559-4502$$aWiggins, Elizabeth$$b4
000916492 7001_ $$00000-0002-3949-6627$$aGargulinski, Emily M.$$b5
000916492 7001_ $$00000-0003-4596-1027$$aShingler, Taylor$$b6
000916492 7001_ $$0P:(DE-HGF)0$$aFenn, Marta$$b7
000916492 7001_ $$00000-0002-4849-9125$$aGriffin, Debora$$b8
000916492 7001_ $$00000-0002-2727-0954$$aHolmes, Christopher D.$$b9
000916492 7001_ $$00000-0001-8558-1294$$aYe, Xinxin$$b10
000916492 7001_ $$00000-0002-3879-7962$$aSaide, Pablo E.$$b11
000916492 7001_ $$00000-0002-2875-1258$$aBourgeois, Ilann$$b12
000916492 7001_ $$00000-0002-9320-7101$$aPeischl, Jeff$$b13
000916492 7001_ $$00000-0002-7101-9054$$aWomack, Caroline C.$$b14
000916492 7001_ $$00000-0002-8106-3702$$aWashenfelder, Rebecca A.$$b15
000916492 7001_ $$00000-0001-7539-353X$$aVeres, Patrick R.$$b16
000916492 7001_ $$00000-0002-3986-1727$$aNeuman, J. Andrew$$b17
000916492 7001_ $$00000-0002-7899-9948$$aGilman, Jessica B.$$b18
000916492 7001_ $$00000-0002-5131-7070$$aLamplugh, Aaron$$b19
000916492 7001_ $$00000-0002-7095-3718$$aSchwantes, Rebecca H.$$b20
000916492 7001_ $$0P:(DE-HGF)0$$aMcKeen, Stuart A.$$b21
000916492 7001_ $$00000-0001-5050-3018$$aWisthaler, Armin$$b22
000916492 7001_ $$00000-0002-8191-8029$$aPiel, Felix$$b23
000916492 7001_ $$00000-0003-0487-3610$$aGuo, Hongyu$$b24
000916492 7001_ $$00000-0003-3930-010X$$aCampuzano-Jost, Pedro$$b25
000916492 7001_ $$00000-0001-6203-1847$$aJimenez, Jose L.$$b26
000916492 7001_ $$0P:(DE-HGF)0$$aFried, Alan$$b27
000916492 7001_ $$00000-0001-9434-8507$$aHanisco, Thomas F.$$b28
000916492 7001_ $$00000-0002-0518-7690$$aHuey, Lewis Gregory$$b29
000916492 7001_ $$00000-0003-2231-7503$$aPerring, Anne$$b30
000916492 7001_ $$0P:(DE-HGF)0$$aKatich, Joseph M.$$b31
000916492 7001_ $$00000-0002-3617-0269$$aDiskin, Glenn S.$$b32
000916492 7001_ $$00000-0002-5697-9807$$aNowak, John B.$$b33
000916492 7001_ $$00000-0001-9189-0405$$aBui, T. Paul$$b34
000916492 7001_ $$00000-0001-9499-9836$$aHalliday, Hannah S.$$b35
000916492 7001_ $$00000-0002-6764-8624$$aDiGangi, Joshua P.$$b36
000916492 7001_ $$00000-0002-2093-9942$$aPereira, Gabriel$$b37
000916492 7001_ $$00000-0002-6507-4997$$aJames, Eric P.$$b38
000916492 7001_ $$00000-0002-6996-7071$$aAhmadov, Ravan$$b39
000916492 7001_ $$00000-0001-5054-1380$$aMcLinden, Chris A.$$b40
000916492 7001_ $$00000-0001-8637-3040$$aSoja, Amber J.$$b41
000916492 7001_ $$00000-0003-2911-4469$$aMoore, Richard H.$$b42
000916492 7001_ $$00000-0002-9672-1237$$aHair, Johnathan W.$$b43
000916492 7001_ $$00000-0003-3811-8496$$aWarneke, Carsten$$b44
000916492 773__ $$0PERI:(DE-600)1465132-4$$a10.1021/acs.est.1c07121$$gVol. 56, no. 12, p. 7564 - 7577$$n12$$p7564 - 7577$$tEnvironmental science & technology$$v56$$x0013-936X$$y2022
000916492 8564_ $$uhttps://juser.fz-juelich.de/record/916492/files/acs.est.1c07121-1.pdf$$yRestricted
000916492 8564_ $$uhttps://juser.fz-juelich.de/record/916492/files/Stockwell_ES%26T.pdf$$yPublished on 2022-05-17. Available in OpenAccess from 2023-05-17.
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