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@ARTICLE{Stockwell:916492,
author = {Stockwell, Chelsea E. and Bela, Megan M. and Coggon,
Matthew M. and Gkatzelis, Georgios and Wiggins, Elizabeth
and Gargulinski, Emily M. and Shingler, Taylor and Fenn,
Marta and Griffin, Debora and Holmes, Christopher D. and Ye,
Xinxin and Saide, Pablo E. and Bourgeois, Ilann and Peischl,
Jeff and Womack, Caroline C. and Washenfelder, Rebecca A.
and Veres, Patrick R. and Neuman, J. Andrew and Gilman,
Jessica B. and Lamplugh, Aaron and Schwantes, Rebecca H. and
McKeen, Stuart A. and Wisthaler, Armin and Piel, Felix and
Guo, Hongyu and Campuzano-Jost, Pedro and Jimenez, Jose L.
and Fried, Alan and Hanisco, Thomas F. and Huey, Lewis
Gregory and Perring, Anne and Katich, Joseph M. and Diskin,
Glenn S. and Nowak, John B. and Bui, T. Paul and Halliday,
Hannah S. and DiGangi, Joshua P. and Pereira, Gabriel and
James, Eric P. and Ahmadov, Ravan and McLinden, Chris A. and
Soja, Amber J. and Moore, Richard H. and Hair, Johnathan W.
and Warneke, Carsten},
title = {{A}irborne {E}mission {R}ate {M}easurements {V}alidate
{R}emote {S}ensing {O}bservations and {E}mission
{I}nventories of {W}estern {U}.{S}. {W}ildfires},
journal = {Environmental science $\&$ technology},
volume = {56},
number = {12},
issn = {0013-936X},
address = {Columbus, Ohio},
publisher = {American Chemical Society},
reportid = {FZJ-2022-06282},
pages = {7564 - 7577},
year = {2022},
abstract = {Carbonaceous emissions from wildfires are a dynamic mixture
of gases and particles that have important impacts on air
quality and climate. Emissions that feed atmospheric models
are estimated using burned area and fire radiative power
(FRP) methods that rely on satellite products. These
approaches show wide variability and have large
uncertainties, and their accuracy is challenging to evaluate
due to limited aircraft and ground measurements. Here, we
present a novel method to estimate fire plume-integrated
total carbon and speciated emission rates using a unique
combination of lidar remote sensing aerosol extinction
profiles and in situ measured carbon constituents. We show
strong agreement between these aircraft-derived emission
rates of total carbon and a detailed burned area-based
inventory that distributes carbon emissions in time using
Geostationary Operational Environmental Satellite FRP
observations (Fuel2Fire inventory, slope = 1.33 ± 0.04, r2
= 0.93, and RMSE = 0.27). Other more commonly used
inventories strongly correlate with aircraft-derived
emissions but have wide-ranging over- and under-predictions.
A strong correlation is found between carbon monoxide
emissions estimated in situ with those derived from the
TROPOspheric Monitoring Instrument (TROPOMI) for five
wildfires with coincident sampling windows (slope = 0.99 ±
0.18; bias = $28.5\%).$ Smoke emission coefficients (g
MJ–1) enable direct estimations of primary gas and aerosol
emissions from satellite FRP observations, and we derive
these values for many compounds emitted by temperate forest
fuels, including several previously unreported species.},
cin = {IEK-8},
ddc = {333.7},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {2111 - Air Quality (POF4-211)},
pid = {G:(DE-HGF)POF4-2111},
typ = {PUB:(DE-HGF)16},
pubmed = {35579536},
UT = {WOS:000815803000001},
doi = {10.1021/acs.est.1c07121},
url = {https://juser.fz-juelich.de/record/916492},
}