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000943287 1001_ $$0P:(DE-Juel1)190810$$aWeiling, Matthias$$b0
000943287 245__ $$aVibrational Spectroscopy Insight into the Electrode|electrolyte Interface/Interphase in Lithium Batteries
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000943287 520__ $$aLithium-ion batteries (LIBs) have transformed the use of mobile electronics and storage technologies. Alongside advances in materials, an in-depth understanding of the interfacial phenomena and interphase formation mechanisms in LIBs is crucial. Interphases are widely recognized as the most important and the least understood components of LIBs and play a direct role in defining cell performance, cyclability, and safety. This article presents a review of recent developments in vibrational spectroscopy techniques of Raman, infrared, and sum-frequency generation spectroscopies to probe the fundamental aspects of interphases on the anode and cathode of LIBs. First the vibrational spectroscopy techniques and their relevant technical considerations for interphase characterization are briefly introduced. In the next step, the latest studies on the fundamental properties, composition, and structure of interphases employing vibrational spectroscopy techniques are presented. This review focuses on in situ/operando investigations; however, post-mortem studies are also discussed briefly.
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000943287 536__ $$0G:(BMBF)13XP5129$$aElektrolytformulierungen für Lithiumbatterien der nächsten Generation mit großer Energiedichte und hoher Beständigkeit (13XP5129)$$c13XP5129$$x1
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000943287 7001_ $$0P:(DE-Juel1)188450$$aPfeiffer, Felix$$b1
000943287 7001_ $$00000-0002-2754-6623$$aBaghernejad, Masoud$$b2$$eCorresponding author
000943287 773__ $$0PERI:(DE-600)2594556-7$$a10.1002/aenm.202202504$$gVol. 12, no. 46, p. 2202504 -$$n46$$p2202504 -$$tAdvanced energy materials$$v12$$x1614-6832$$y2022
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