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@ARTICLE{Hamill:943288,
      author       = {Hamill, Joseph and Zhour, Kazem and Diddens, Diddo and
                      Baghernejad, Masoud},
      title        = {{S}ignificant two-step potential-induced surface
                      reconstruction observed on {A}u(1 1 1) in aqueous sulfuric
                      acid},
      journal      = {Electrochemistry communications},
      volume       = {140},
      issn         = {1388-2481},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier Science},
      reportid     = {FZJ-2023-00898},
      pages        = {107332},
      year         = {2022},
      abstract     = {We report in this communication, through in situ STM images
                      correlated with time, and ab initio simulations of binding
                      energies, how potential-induced surface reconstruction is
                      formed on Au(1 1 1) single crystal in 0.1 M H2SO4. It was
                      found that while the electrode potential after lifting the
                      reconstructed surface is switched back to a more negative
                      value than the potential of zero charge, the formation
                      process of the reconstructed surface goes through two
                      consecutive routes. In the more kinetically favorable step,
                      and within a few minutes, the reconstructed surface follows
                      three different lattice directions with a high proportion of
                      semi zig-zag structures. However, by maintaining the
                      negative applied potential, the surface reconstruction
                      rearranges to a straighter reconstructed pattern in the
                      second step, which is more energetically favorable.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) /
                      Elektrolytformulierungen für Lithiumbatterien der nächsten
                      Generation mit großer Energiedichte und hoher
                      Beständigkeit (13XP5129)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(BMBF)13XP5129},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000891239800002},
      doi          = {10.1016/j.elecom.2022.107332},
      url          = {https://juser.fz-juelich.de/record/943288},
}