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| Home > Publications database > Significant two-step potential-induced surface reconstruction observed on Au(1 1 1) in aqueous sulfuric acid > print |
| 001 | 943288 | ||
| 005 | 20240712113111.0 | ||
| 024 | 7 | _ | |a 10.1016/j.elecom.2022.107332 |2 doi |
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| 037 | _ | _ | |a FZJ-2023-00898 |
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| 100 | 1 | _ | |a Hamill, Joseph |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Significant two-step potential-induced surface reconstruction observed on Au(1 1 1) in aqueous sulfuric acid |
| 260 | _ | _ | |a Amsterdam [u.a.] |c 2022 |b Elsevier Science |
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| 520 | _ | _ | |a We report in this communication, through in situ STM images correlated with time, and ab initio simulations of binding energies, how potential-induced surface reconstruction is formed on Au(1 1 1) single crystal in 0.1 M H2SO4. It was found that while the electrode potential after lifting the reconstructed surface is switched back to a more negative value than the potential of zero charge, the formation process of the reconstructed surface goes through two consecutive routes. In the more kinetically favorable step, and within a few minutes, the reconstructed surface follows three different lattice directions with a high proportion of semi zig-zag structures. However, by maintaining the negative applied potential, the surface reconstruction rearranges to a straighter reconstructed pattern in the second step, which is more energetically favorable. |
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| 700 | 1 | _ | |a Baghernejad, Masoud |0 P:(DE-HGF)0 |b 3 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.elecom.2022.107332 |g Vol. 140, p. 107332 - |0 PERI:(DE-600)2027290-X |p 107332 |t Electrochemistry communications |v 140 |y 2022 |x 1388-2481 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/943288/files/1-s2.0-S1388248122001345-main.pdf |y OpenAccess |
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