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000943413 0247_ $$2doi$$a10.1126/sciadv.abn6129
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000943413 1001_ $$0P:(DE-Juel1)171614$$aHouston, Judith Elizabeth$$b0
000943413 245__ $$aResolving the different bulk moduli within individual soft nanogels using small-angle neutron scattering
000943413 260__ $$aWashington, DC [u.a.]$$bAssoc.$$c2022
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000943413 520__ $$aThe bulk modulus, K, quantifies the elastic response of an object to an isotropic compression. For soft compressible colloids, knowing K is essential to accurately predict the suspension response to crowding. Most colloids have complex architectures characterized by different softness, which additionally depends on compression. Here, we determine the different values of K for the various morphological parts of individual nanogels and probe the changes of K with compression. Our method uses a partially deuterated polymer, which exerts the required isotropic stress, and small-angle neutron scattering with contrast matching to determine the form factor of the particles without any scattering contribution from the polymer. We show a clear difference in softness, compressibility, and evolution of K between the shell of the nanogel and the rest of the particle, depending on the amount of cross-linker used in their synthesis.
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000943413 7001_ $$0P:(DE-Juel1)169361$$aFruhner, Lisa$$b1
000943413 7001_ $$0P:(DE-HGF)0$$ade la Cotte, Alexis$$b2
000943413 7001_ $$0P:(DE-HGF)0$$aRojo González, Javier$$b3
000943413 7001_ $$0P:(DE-HGF)0$$aPetrunin, Alexander Valerievich$$b4
000943413 7001_ $$0P:(DE-HGF)0$$aGasser, Urs$$b5
000943413 7001_ $$0P:(DE-HGF)0$$aSchweins, Ralf$$b6
000943413 7001_ $$0P:(DE-Juel1)130501$$aAllgaier, J.$$b7$$ufzj
000943413 7001_ $$0P:(DE-Juel1)IHRS-BioSoft-140012$$aRichtering, Walter$$b8
000943413 7001_ $$0P:(DE-HGF)0$$aFernandez-Nieves, Alberto$$b9
000943413 7001_ $$0P:(DE-HGF)0$$aScotti, Andrea$$b10$$eCorresponding author
000943413 773__ $$0PERI:(DE-600)2810933-8$$a10.1126/sciadv.abn6129$$gVol. 8, no. 26, p. eabn6129$$n26$$peabn6129$$tScience advances$$v8$$x2375-2548$$y2022
000943413 8564_ $$uhttps://juser.fz-juelich.de/record/943413/files/sciadv.abn6129.pdf$$yOpenAccess
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