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@ARTICLE{Hendriks:943461,
      author       = {Hendriks, Theodoor Anton and Lange, Martin and Kiens, Ellen
                      and Baeumer, Christoph and Zeier, Wolfgang},
      title        = {{B}alancing {P}artial {I}onic and {E}lectronic {T}ransport
                      for {O}ptimized {C}athode {U}tilization of {H}igh‐voltage
                      ${L}i{M}n_2{O}_4 / {L}i_3{I}n{C}l_6$ {S}olid‐state
                      {B}atteries},
      journal      = {Batteries $\&$ supercaps},
      volume       = {6},
      number       = {4},
      issn         = {2566-6223},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2023-01032},
      pages        = {e202200544},
      year         = {2023},
      abstract     = {Their suggested stability towards high-voltage cathode
                      materials makes halide-based solid electrolytes currently an
                      interesting class of ionic conductors for solid-state
                      batteries. Especially the LiMn2O4 spinel cathode active
                      material is of interest due to its slightly higher nominal
                      voltage and more resilience to overcharging compared to
                      LiCoO2 and LiNixMnyCozO2 cathodes. Typically, a standard
                      ratio of active material to solid electrolyte is used in
                      composites for solid-state batteries. However, for ideal
                      transport properties, and thus to achieve balanced and
                      optimal partial-conductivities, this ratio needs to be
                      re-optimized each time the material basis is changed. In
                      this work, we show transport in the composite measured
                      through both DC polarization as well as transmission line
                      modeling of the impedance spectra. By balancing the partial
                      transport parameters of the composite, an optimum capacity
                      of the solid-state batteries is achieved. This work shows
                      characterization and optimization of transport is required
                      for unlocking the full potential of solid-state batteries.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000929056700001},
      doi          = {10.1002/batt.202200544},
      url          = {https://juser.fz-juelich.de/record/943461},
}