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000009699 084__ $$2WoS$$aPhysics, Multidisciplinary
000009699 1001_ $$0P:(DE-HGF)0$$aMartin, J.$$b0
000009699 245__ $$aDirect Observation of confined Single Chain Dynamics by Neutron Scattering
000009699 260__ $$aCollege Park, Md.$$bAPS$$c2010
000009699 300__ $$a197801
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000009699 440_0 $$04925$$aPhysical Review Letters$$v104$$x0031-9007$$y19
000009699 500__ $$aWe thank M. Hernandez-Velez, A. R. Gonzalez-Elipe, J. Gil, R. Sastre, O. Garcia, and M. Brodeck, SoftComp NoE, MAT2007-63681, IT-436-07 (GV), the MEyC (CSD2006-53), Grants FPU AP2005-1063 and MAT2008-1073.
000009699 520__ $$aNeutron spin echo has revealed the single chain dynamic structure factor of entangled polymer chains confined in cylindrical nanopores with chain dimensions either much larger or smaller than the lateral pore sizes. In both situations, a slowing down of the dynamics with respect to the bulk behavior is only observed at intermediate times. The results at long times provide a direct microscopic measurement of the entanglement distance under confinement. They constitute the first experimental microscopic evidence of the dilution of the total entanglement density in a polymer melt under strong confinement, a phenomenon that so far was hypothesized on the basis of various macroscopic observations.
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000009699 693__ $$0EXP:(DE-MLZ)KWS2-20140101$$1EXP:(DE-MLZ)FRMII-20140101$$5EXP:(DE-MLZ)KWS2-20140101$$6EXP:(DE-MLZ)NL3ao-20140101$$aForschungs-Neutronenquelle Heinz Maier-Leibnitz$$eKWS-2: Small angle scattering diffractometer$$fNL3ao$$x1
000009699 7001_ $$0P:(DE-Juel1)VDB89817$$aKrutyeva, M.$$b1$$uFZJ
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000009699 7001_ $$0P:(DE-HGF)0$$aMaiz, J.$$b7
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000009699 8567_ $$uhttp://dx.doi.org/10.1103/PhysRevLett.104.197801
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