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| 024 | 7 | _ | |a 10.1524/ract.2010.1708 |2 DOI |
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| 041 | _ | _ | |a eng |
| 082 | _ | _ | |a 540 |
| 084 | _ | _ | |2 WoS |a Chemistry, Inorganic & Nuclear |
| 084 | _ | _ | |2 WoS |a Nuclear Science & Technology |
| 100 | 1 | _ | |0 P:(DE-Juel1)130383 |a Modolo, G. |b 0 |u FZJ |
| 245 | _ | _ | |a Demonstration of the LUCA process for the separation of americium(III) from curium(III), californium(III), and lanthanides(III) in acidic solution using a synergistic mixture of bis(chlorophenyl)dithiophosphinic acid and tris(2-ethylhexyl)phosphate |
| 260 | _ | _ | |a München |b Oldenbourg |c 2010 |
| 300 | _ | _ | |a 193 - 201 |
| 336 | 7 | _ | |a Journal Article |0 PUB:(DE-HGF)16 |2 PUB:(DE-HGF) |
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| 440 | _ | 0 | |0 5243 |a Radiochimica Acta |v 98 |x 0033-8230 |y 4 |
| 500 | _ | _ | |a Financial support for this research was provided by the European Commission (project ACSEPT No. 211267). |
| 520 | _ | _ | |a The LUCA process was developed at Forschungszentrum Julich for the selective separation of Am(III) from an acidic solution containing the trivalent actinides Am(III). Cm(III), and Cf(III) as well as lanthanides. A mixture of 0.4 mol/L bis(chlorophenyl)dithiophosphinic acid and 0.15 mol/L tris(2-ethylhexyl)phosphate dissolved in 20% isooctane/80% tert-butyl benzene was used as the extractant. The process was carried out in centrifugal contactors using an optimized flowsheet involving 7 stages for extraction, 9 stages for scrubbing and 8 stages for back-extraction. Very encouraging results were obtained. A high feed decontamination factor was obtained for Am(III) (> 1000), and recovery in the product after stripping was higher than 99.8%. The Am(III) product was contaminated with 0.47% Cm(III). More than 99.9% Cf(III), Eu(III) and > 99.5% Cm(III) inventories were directed to the raffinate and the contamination with Am(III) (< 0.08%) was low. The experimental results were in good agreement with the predictions of a computer code. |
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| 536 | _ | _ | |0 G:(EU-Grant)211267 |a ACSEPT - Actinide reCycling by SEParation and Transmutation (211267) |c 211267 |f FP7-Fission-2007 |x 1 |
| 588 | _ | _ | |a Dataset connected to Web of Science |
| 650 | _ | 7 | |2 WoSType |a J |
| 653 | 2 | 0 | |2 Author |a Minor actinides |
| 653 | 2 | 0 | |2 Author |a Lanthanides |
| 653 | 2 | 0 | |2 Author |a Americium |
| 653 | 2 | 0 | |2 Author |a Curium |
| 653 | 2 | 0 | |2 Author |a Partitioning |
| 653 | 2 | 0 | |2 Author |a Solvent extraction |
| 653 | 2 | 0 | |2 Author |a Centrifugal contactors |
| 653 | 2 | 0 | |2 Author |a LUCA process |
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| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Geist, A. |b 2 |
| 773 | _ | _ | |0 PERI:(DE-600)2039575-9 |a 10.1524/ract.2010.1708 |g Vol. 98, p. 193 - 201 |p 193 - 201 |q 98<193 - 201 |t Radiochimica acta |v 98 |x 0033-8230 |y 2010 |
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