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000009932 084__ $$2WoS$$aPhysics, Fluids & Plasmas
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000009932 1001_ $$0P:(DE-HGF)0$$aLe Coeur, C.$$b0
000009932 245__ $$aCompression of random coils due to macromolecular crowding: Scaling effects
000009932 260__ $$aCollege Park, Md.$$bAPS$$c2010
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000009932 520__ $$aThe addition of a macromolecular crowding agent to a dilute solution of polymer exerts a compressive force that tends to reduce the size of the chain. We study here the effect of changing the size ratio between the random coil and the crowding agent. The compression occurs at lower crowding agent concentration, Phi when polymer molecular weight increases. The Flory exponent nu(Phi) decreases from nu(0)similar or equal to 0.48 in water down to 0.3 with macromolecular crowding. The effective polymer-polymer interactions change from repulsive to strongly attractive inducing aggregation of the chains. This effect changes drastically for larger polymer sizes, being much more pronounced at high molecular weights.
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000009932 8567_ $$uhttp://dx.doi.org/10.1103/PhysRevE.81.061914
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