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Diamond is a promising platform for quantum information processing as it can host highly coherent qubits that could allow for the construction of large quantum registers. A prerequisite for such devices is a coherent interaction between nitrogen-vacancy (NV) electron spins enabling scalable entanglement. [...]

Projected entangled pair states (PEPS) on finite two-dimensional lattices are a natural ansatz for representing ground states of local many-body Hamiltonians, as they inherently satisfy the boundary law of entanglement entropy. In this paper, we propose the optimization of PEPS via an improved formulation of the time-dependent variational principle (TDVP), namely the minimum-step stochastic-reconfiguration scheme recently introduced for neural quantum states. [...]