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@ARTICLE{Weber:1005795,
      author       = {Weber, Felix M. and Graff, Karl Martin and Kohlhaas, Ina
                      and Figgemeier, Egbert},
      title        = {{E}ffective {L}ithium {P}assivation through {G}raphite
                      {C}oating for {L}ithium {M}etal {B}atteries},
      journal      = {ACS applied energy materials},
      volume       = {6},
      number       = {6},
      issn         = {2574-0962},
      address      = {Washington, DC},
      publisher    = {ACS Publications},
      reportid     = {FZJ-2023-01640},
      pages        = {3413 - 3421},
      year         = {2023},
      abstract     = {Metallic lithium reacts with organic solvents, resulting in
                      their decomposition. The prevention of these decomposition
                      reactions is a key aspect enabling the use of metallic
                      lithium as an anode in lithium metal batteries. Scanning
                      electrochemical microscopy (SECM), laser microscopy, and
                      Fourier transform infrared (FT-IR) spectroscopy were used to
                      analyze the effect of a graphite coating on metallic
                      lithium. The graphite layer successfully prevents the
                      agglomeration of decomposition products on the surface. SECM
                      data show that the surface of untreated lithium metal in
                      electrolyte is insulating, but the surface of the graphite
                      coated lithium appears conducting and is therefore not
                      covered by any layer of decomposition products. The
                      protective properties of the graphite layer were proofed
                      using FT-IR data. No significant differences in the spectra
                      evolved during immersion of the sample in the electrolyte.
                      Electrochemical plating experiments and post-mortem analysis
                      revealed that the graphite layer did not result in
                      homogeneous lithium plating depending on the current
                      density. At high currents, no fully covering layer of
                      decomposition products was formed on the surface during
                      plating experiments, indicating a more complex mechanism of
                      solid–electrolyte interface formation.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / Lillint -
                      Thermodynamic and kinetic stability of the Lithium-Liquid
                      Electrolyte Interface (13XP0225B)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(BMBF)13XP0225B},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000959225800001},
      doi          = {10.1021/acsaem.2c04128},
      url          = {https://juser.fz-juelich.de/record/1005795},
}