Home > Workflow collections > Publication Charges > Aqueous Processing of LiCoO 2 –Li 6.6 La 3 Zr 1.6 Ta 0.4 O 12 Composite Cathode for High-Capacity Solid-State Lithium Batteries > print

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100 1 _ |a Ye, Ruijie
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245 _ _ |a Aqueous Processing of LiCoO 2 –Li 6.6 La 3 Zr 1.6 Ta 0.4 O 12 Composite Cathode for High-Capacity Solid-State Lithium Batteries
260 _ _ |a Washington, DC
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520 _ _ |a To fabricate ceramic composite cathodes LiCoO2–Li6.6La3Zr1.6Ta0.4O12 (LCO-LLZTO) on an industrial scale, a water-based tape-casting process was developed, which is scalable and environmentally friendly. Additionally, the cosintering behavior of the two materials, often leading to poor electrochemical performance, was optimized via a Li2O-rich atmosphere. The resulting dense, free-standing, and phase-pure LCO-LLZTO mixed cathodes were assembled into full cells using a dual-layer solid polymer-ceramic separator and an In–Li anode. These cells show very high utilization rates for LCO of approximately 90% at a high areal capacity of over 3 mAh cm–2, demonstrating the potential of water-based tape-casting for a scalable and sustainable manufacturing of oxide-ceramic based solid-state Li batteries.
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700 1 _ |a Ihrig, Martin
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700 1 _ |a Figgemeier, Egbert
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700 1 _ |a Fattakhova-Rohlfing, Dina
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700 1 _ |a Finsterbusch, Martin
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773 _ _ |a 10.1021/acssuschemeng.2c07556
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