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@ARTICLE{Yu:1007368,
author = {Yu, Shangzhe and Zhang, Shidong and Schäfer, Dominik and
Peters, Roland and Kunz, Felix and Eichel, Rüdiger-A.},
title = {{N}umerical {M}odeling and {S}imulation of the {S}olid
{O}xide {C}ell {S}tacks and {M}etal {I}nterconnect
{O}xidation with {O}pen{FOAM}},
journal = {Energies},
volume = {16},
number = {9},
issn = {1996-1073},
address = {Basel},
publisher = {MDPI},
reportid = {FZJ-2023-02033},
pages = {3827 -},
year = {2023},
abstract = {Solid oxide cells are capable of efficiently converting
various chemical energy carriers to electricity and vice
versa. The urgent challenge nowadays is the faster
degradation rate compared with other fuel cell/electrolyzer
technologies. To understand the degradation mechanisms,
simulation of a solid oxide cell is helpful. Since most
previous research developed models using commercial
software, such as COMSOL and ANSYS Fluent, a gap for
knowledge transfer is being gradually formed between
academia and industry due to licensing issues. This paper
introduces a multiphysics model, developed by a
computational code, openFuelCell2. The code is implemented
with an open-source library, OpenFOAM. It accounts for
momentum transfer, mass transfer, electrochemical reactions
and metal interconnect oxidation. The model can precisely
predict I–V curves under different temperatures, fuel
humidity and operation modes. Comparison between OpenFOAM
and COMSOL simulations shows good agreement. The metal
interconnect oxidation is modeled, which can predict the
thickness of the oxide scale under different protective
coatings. Simulations are conducted by assuming an
ultra-thin film resistance on the rib surface. It is
revealed that coatings fabricated by atmospheric plasma
spraying can efficiently prevent metal interconnect
oxidation, with a contribution of only 0.53 $\%$ to the
total degradation rate.},
cin = {IEK-9},
ddc = {620},
cid = {I:(DE-Juel1)IEK-9-20110218},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123) / HITEC -
Helmholtz Interdisciplinary Doctoral Training in Energy and
Climate Research (HITEC) (HITEC-20170406) / Verbundvorhaben
$SOC-Degradation_2$ ' Teilvorhaben A (03SF0621A)},
pid = {G:(DE-HGF)POF4-1231 / G:(DE-Juel1)HITEC-20170406 /
G:(BMBF)03SF0621A},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000987332400001},
doi = {10.3390/en16093827},
url = {https://juser.fz-juelich.de/record/1007368},
}