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@ARTICLE{Chen:1007380,
      author       = {Chen, Yi-Hsuan and Lennartz, Peter and Liu, Kun Ling and
                      Hsieh, Yi-Chen and Scharf, Felix and Guerdelli, Rayan and
                      Buchheit, Annika and Grünebaum, Mariano and Kempe, Fabian
                      and Winter, Martin and Brunklaus, Gunther},
      title        = {{T}owards {A}ll‐{S}olid‐{S}tate {P}olymer {B}atteries:
                      {G}oing {B}eyond {PEO} with {H}ybrid {C}oncepts},
      journal      = {Advanced functional materials},
      volume       = {33},
      number       = {32},
      issn         = {1616-301X},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2023-02045},
      pages        = {2300501},
      year         = {2023},
      abstract     = {To go beyond polyethylene oxide in lithium metal batteries,
                      a hybrid polymer/oligomer cell design is presented, where an
                      ester oligomer provides high ionic conductivity of 0.2 mS
                      cm−1 at 40 °C within thicker composite cathodes with
                      active mass loadings of up to 11 mg cm−2 (LiNbO3-coated)
                      LiNi0.6Mn0.2Co0.2 (NMC622), while a 30 µm thin
                      scaffold-supported polymer electrolyte affords mechanical
                      stability. Corresponding discharge capacities of the hybrid
                      cells exceed 170 mAh g−1 (11 mg cm−2) or 160 mAh g−1
                      (6 mg cm−2) at rates of either 0.1 or 0.25 C. Multilayer
                      pouch cells are projected to enable energy densities of 235
                      Wh L−1 (6 mg cm−2) and even up to 356 Wh L−1 (11 mg
                      cm−2), clearly superior to other reported polymer-based
                      cell designs. Polyester electrolytes are environmentally
                      benign and safer compared to common liquid electrolytes,
                      while the straightforward synthesis and affordability of
                      precursors render hybrid polyester electrolytes suitable
                      candidates for future application in solid-state lithium
                      metal batteries.},
      cin          = {IEK-12},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / 1222 -
                      Components and Cells (POF4-122) / 1223 - Batteries in
                      Application (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(DE-HGF)POF4-1222 /
                      G:(DE-HGF)POF4-1223},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000975115700001},
      doi          = {10.1002/adfm.202300501},
      url          = {https://juser.fz-juelich.de/record/1007380},
}