Home > Workflow collections > Publication Charges > Bimetallic Copper–Silver Catalysts for the Electrochemical Reduction of CO 2 to Ethanol > print

001     1009254
005     20240712112835.0
024 7 _ |a 10.1021/acsaem.3c00985
|2 doi
024 7 _ |a 10.34734/FZJ-2023-02714
|2 datacite_doi
024 7 _ |a WOS:001027010900001
|2 WOS
037 _ _ |a FZJ-2023-02714
082 _ _ |a 540
100 1 _ |a Robens, Elisabeth
|0 P:(DE-Juel1)180626
|b 0
|e Corresponding author
245 _ _ |a Bimetallic Copper–Silver Catalysts for the Electrochemical Reduction of CO 2 to Ethanol
260 _ _ |a Washington, DC
|c 2023
|b ACS Publications
336 7 _ |a article
|2 DRIVER
336 7 _ |a Output Types/Journal article
|2 DataCite
336 7 _ |a Journal Article
|b journal
|m journal
|0 PUB:(DE-HGF)16
|s 1698384282_23571
|2 PUB:(DE-HGF)
336 7 _ |a ARTICLE
|2 BibTeX
336 7 _ |a JOURNAL_ARTICLE
|2 ORCID
336 7 _ |a Journal Article
|0 0
|2 EndNote
520 _ _ |a The electrochemical reduction of carbon dioxide to ethanol is a promising way to make CO2 electrolysis economically feasible. In this work, a bimetallic catalyst of silver and copper is synthesized, and the effect of its copper content on the formation of ethanol is analyzed. By decreasing the near-surface copper content from 99 to 45% (measured by XPS) at a current density of −20 mA cm–2, the Faradaic efficiency of ethanol could be enhanced from 5 to 23%. Moreover, we show that with excess of CO, due to a lower copper and a higher silver near-surface content, the formation of ethanol is favored over ethylene.
536 _ _ |a 1221 - Fundamentals and Materials (POF4-122)
|0 G:(DE-HGF)POF4-1221
|c POF4-122
|f POF IV
|x 0
536 _ _ |a 1232 - Power-based Fuels and Chemicals (POF4-123)
|0 G:(DE-HGF)POF4-1232
|c POF4-123
|f POF IV
|x 1
536 _ _ |a HITEC - Helmholtz Interdisciplinary Doctoral Training in Energy and Climate Research (HITEC) (HITEC-20170406)
|0 G:(DE-Juel1)HITEC-20170406
|c HITEC-20170406
|x 2
536 _ _ |a iNEW2.0 (BMBF-03SF0627A)
|0 G:(DE-Juel1)BMBF-03SF0627A
|c BMBF-03SF0627A
|x 3
588 _ _ |a Dataset connected to CrossRef, Journals: juser.fz-juelich.de
700 1 _ |a Hecker, Burkhard
|0 P:(DE-Juel1)179451
|b 1
700 1 _ |a Kungl, Hans
|0 P:(DE-Juel1)157700
|b 2
700 1 _ |a Tempel, Hermann
|0 P:(DE-Juel1)161208
|b 3
700 1 _ |a Eichel, Rüdiger-A.
|0 P:(DE-Juel1)156123
|b 4
773 _ _ |a 10.1021/acsaem.3c00985
|g p. acsaem.3c00985
|0 PERI:(DE-600)2916551-9
|n 14
|p 7571–7577
|t ACS applied energy materials
|v 6
|y 2023
|x 2574-0962
856 4 _ |u https://juser.fz-juelich.de/record/1009254/files/robens-et-al-2023-bimetallic-copper-silver-catalysts-for-the-electrochemical-reduction-of-co2-to-ethanol.pdf
|y OpenAccess
909 C O |o oai:juser.fz-juelich.de:1009254
|p openaire
|p open_access
|p driver
|p VDB
|p openCost
|p dnbdelivery
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 0
|6 P:(DE-Juel1)180626
910 1 _ |a RWTH Aachen
|0 I:(DE-588b)36225-6
|k RWTH
|b 0
|6 P:(DE-Juel1)180626
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 1
|6 P:(DE-Juel1)179451
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 2
|6 P:(DE-Juel1)157700
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 3
|6 P:(DE-Juel1)161208
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 4
|6 P:(DE-Juel1)156123
910 1 _ |a RWTH Aachen
|0 I:(DE-588b)36225-6
|k RWTH
|b 4
|6 P:(DE-Juel1)156123
913 1 _ |a DE-HGF
|b Forschungsbereich Energie
|l Materialien und Technologien für die Energiewende (MTET)
|1 G:(DE-HGF)POF4-120
|0 G:(DE-HGF)POF4-122
|3 G:(DE-HGF)POF4
|2 G:(DE-HGF)POF4-100
|4 G:(DE-HGF)POF
|v Elektrochemische Energiespeicherung
|9 G:(DE-HGF)POF4-1221
|x 0
913 1 _ |a DE-HGF
|b Forschungsbereich Energie
|l Materialien und Technologien für die Energiewende (MTET)
|1 G:(DE-HGF)POF4-120
|0 G:(DE-HGF)POF4-123
|3 G:(DE-HGF)POF4
|2 G:(DE-HGF)POF4-100
|4 G:(DE-HGF)POF
|v Chemische Energieträger
|9 G:(DE-HGF)POF4-1232
|x 1
914 1 _ |y 2023
915 p c |a APC keys set
|0 PC:(DE-HGF)0000
|2 APC
915 p c |a Helmholtz: American Chemical Society 01/01/2023
|0 PC:(DE-HGF)0122
|2 APC
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0200
|2 StatID
|b SCOPUS
|d 2023-08-25
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0160
|2 StatID
|b Essential Science Indicators
|d 2023-08-25
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)1160
|2 StatID
|b Current Contents - Engineering, Computing and Technology
|d 2023-08-25
915 _ _ |a Creative Commons Attribution CC BY 4.0
|0 LIC:(DE-HGF)CCBY4
|2 HGFVOC
915 _ _ |a JCR
|0 StatID:(DE-HGF)0100
|2 StatID
|b ACS APPL ENERG MATER : 2022
|d 2023-08-25
915 _ _ |a IF >= 5
|0 StatID:(DE-HGF)9905
|2 StatID
|b ACS APPL ENERG MATER : 2022
|d 2023-08-25
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0150
|2 StatID
|b Web of Science Core Collection
|d 2023-08-25
915 _ _ |a WoS
|0 StatID:(DE-HGF)0113
|2 StatID
|b Science Citation Index Expanded
|d 2023-08-25
915 _ _ |a OpenAccess
|0 StatID:(DE-HGF)0510
|2 StatID
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)1150
|2 StatID
|b Current Contents - Physical, Chemical and Earth Sciences
|d 2023-08-25
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0300
|2 StatID
|b Medline
|d 2023-08-25
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0199
|2 StatID
|b Clarivate Analytics Master Journal List
|d 2023-08-25
920 _ _ |l yes
920 1 _ |0 I:(DE-Juel1)IEK-9-20110218
|k IEK-9
|l Grundlagen der Elektrochemie
|x 0
980 1 _ |a APC
980 1 _ |a FullTexts
980 _ _ |a journal
980 _ _ |a VDB
980 _ _ |a UNRESTRICTED
980 _ _ |a I:(DE-Juel1)IEK-9-20110218
980 _ _ |a APC
981 _ _ |a I:(DE-Juel1)IET-1-20110218

LibraryCollectionCLSMajorCLSMinorLanguageAuthor
Marc 21