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001009338 1001_ $$0P:(DE-Juel1)174238$$aRan, Ke$$b0$$eCorresponding author
001009338 245__ $$aDirect Visualization of Distorted Twin Boundaries in Ce-Doped GdFeO3
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001009338 520__ $$aUtilizing advanced transmission electron microscopy (TEM), the structure at the (110)-type twin boundary (TB) of Ce-doped GdFeO3 (C-GFO) has been investigated with picometer precision. Such a TB is promising to generate local ferroelectricity within a paraelectric system, while precise knowledge about its structure is still largely missing. In this work, a direct measurement of the cation off-centering with respect to the neighboring oxygen is enabled by integrated differential phase contrast (iDPC) imaging, and up to 30 pm Gd off-centering is highly localized at the TB. Further electron energy loss spectroscopy (EELS) analysis demonstrates a slight accumulation of oxygen vacancies at the TB, a self-balanced behavior of Ce at the Gd sites, and a mixed occupation of Fe2+ and Fe3+ at the Fe sites. Our results provide an informative picture with atomic details at the TB of C-GFO, which is indispensable to further push the potential of grain boundary engineering.
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001009338 7001_ $$0P:(DE-Juel1)130525$$aBarthel, Juri$$b1
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001009338 7001_ $$0P:(DE-Juel1)180325$$aBuchheit, Annika$$b4
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001009338 7001_ $$0P:(DE-Juel1)129587$$aBaumann, Stefan$$b6
001009338 7001_ $$0P:(DE-Juel1)129637$$aMeulenberg, Wilhelm Albert$$b7
001009338 7001_ $$0P:(DE-Juel1)130824$$aMayer, Joachim$$b8
001009338 773__ $$0PERI:(DE-600)2048866-X$$a10.1021/acs.nanolett.3c00318$$n7$$p2945-2951$$tNano letters$$v23$$x1530-6984$$y2023
001009338 8564_ $$uhttps://juser.fz-juelich.de/record/1009338/files/Direct%20Visualization.pdf$$yPublished on 2023-03-27. Available in OpenAccess from 2024-03-27.
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