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@ARTICLE{Li:1014720,
      author       = {Li, Chenkun and Peng, Zhangquan and Huang, Jun},
      title        = {{I}mpedance {R}esponse of {E}lectrochemical {I}nterfaces:
                      {P}art {IV}─{L}ow-{F}requency {I}nductive {L}oop for a
                      {S}ingle-{E}lectron {R}eaction},
      journal      = {The journal of physical chemistry / C},
      volume       = {127},
      number       = {33},
      issn         = {1932-7447},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {FZJ-2023-03410},
      pages        = {16367 - 16373},
      year         = {2023},
      abstract     = {The low-frequency inductive loop is usually attributed to
                      relaxation of adsorbed intermediates of multistep reactions
                      in electrocatalysis and corrosion. Herein, we report a
                      low-frequency inductive loop for a single-electron reaction
                      when the electrode potential (EM), the equilibrium potential
                      (Eeq), and the potential of zero charge (Epzc) are
                      different, namely, under nonequilibrium conditions.
                      Interestingly enough, although both reactions involve only
                      one electron, the metal deposition reaction (M+ + e ↔ M)
                      and the redox couple reaction (Fe(CN)63– + e ↔
                      Fe(CN)64–) show different impedance shapes. The
                      low-frequency inductive loop is observed only for the M+ + e
                      ↔ M reaction in the oxidation direction because its
                      faradaic current has a negative phase angle due to double
                      layer effects. Moreover, we find that the low-frequency
                      inductive loop occurs only when the polarization curve has
                      no diffusion-limiting features.},
      cin          = {IEK-13},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-13-20190226},
      pnm          = {1212 - Materials and Interfaces (POF4-121)},
      pid          = {G:(DE-HGF)POF4-1212},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001049424300001},
      doi          = {10.1021/acs.jpcc.3c02830},
      url          = {https://juser.fz-juelich.de/record/1014720},
}