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001014739 1001_ $$0P:(DE-Juel1)159378$$aKegler, Philip$$b0$$eCorresponding author
001014739 245__ $$aAccelerated dissolution of doped UO2-based model systems as analogues for modern spent nuclear fuel under repository conditions
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001014739 520__ $$aSystematic single-effect dissolution studies were carried out on the dissolution behaviour of pure and Cr- or Nd-doped UO2 reference pellets as model materials for spent nuclear fuel with varying doping levels, densities, and grain sizes as well as of industrially produced Cr- and Cr/Nd-doped UO2 pellets. The results were obtained from accelerated static batch dissolution experiments performed under strictly controlled conditions using H2O2 as simulant for radiolytic oxidants formed due to the alpha-irradiation of water. The results indicate that the addition of Cr and the consequential modification of the fuel matrix does not lead to a significant change of the dissolution behaviour of these model materials compared to pure UO2 reference materials. Contrarily, the dissolution rates of Nd-doped pellets are significantly lower than those of pure and Cr-doped pellets. These results provide additional insights into the influence of doping on the dissolution behaviour of modern spent light water reactor fuels under the post-closure conditions expected in a deep geological repository.
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001014739 536__ $$0G:(EU-Grant)755443$$aDISCO - Modern spent fuel dissolution and chemistry in failed container conditions (755443)$$c755443$$fNFRP-2016-2017-1$$x1
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001014739 7001_ $$0P:(DE-Juel1)130389$$aNeumeier, Stefan$$b1
001014739 7001_ $$0P:(DE-Juel1)130364$$aKlinkenberg, Martina$$b2
001014739 7001_ $$0P:(DE-Juel1)130329$$aBukaemskiy, Andrey$$b3
001014739 7001_ $$0P:(DE-Juel1)156511$$aDeissmann, Guido$$b4
001014739 7001_ $$0P:(DE-Juel1)144040$$aBrandt, Felix$$b5
001014739 7001_ $$0P:(DE-Juel1)130324$$aBosbach, Dirk$$b6
001014739 773__ $$0PERI:(DE-600)2858562-8$$a10.1557/s43580-023-00544-y$$gVol. 8, no. 6, p. 255 - 260$$n6$$p255 - 260$$tMRS advances$$v8$$x2059-8521$$y2023
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