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| Hauptseite > Publikationsdatenbank > Design, production, and characterization of three-dimensionally-structured oxide-polymer composite cathodes for all-solid-state batteries > print |
| Hauptseite > Publikationsdatenbank > Design, production, and characterization of three-dimensionally-structured oxide-polymer composite cathodes for all-solid-state batteries > print |
| 001 | 1017752 | ||
| 005 | 20250203103222.0 | ||
| 024 | 7 | _ | |a 10.1016/j.ensm.2023.03.008 |2 doi |
| 024 | 7 | _ | |a 2405-8289 |2 ISSN |
| 024 | 7 | _ | |a 2405-8297 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2023-04288 |
| 082 | _ | _ | |a 624 |
| 100 | 1 | _ | |a Kriegler, Johannes |0 0000-0002-7961-7876 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Design, production, and characterization of three-dimensionally-structured oxide-polymer composite cathodes for all-solid-state batteries |
| 260 | _ | _ | |a Amsterdam |c 2023 |b Elsevier |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1710328103_3657 |2 PUB:(DE-HGF) |
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| 520 | _ | _ | |a Inorganic all-solid-state batteries with oxide electrolytes show improved safety compared to conventional lithium-ion batteries due to the application of a non-flammable solid electrolyte. However, the currently applied production methods are unsuitable for creating oxide composite cathodes with a good interfacial contact between the solid electrolyte and the cathode active material, which limits the accessible discharge capacity. Thus, solid electrolyte matrix-supported all-solid-state batteries, for which a porous scaffold is filled with cathode active material, have recently seen increasing research interest. This publication introduces a scalable production route for a matrix-supported cell concept with a three-dimensionally-structured oxide-based composite cathode. Directed microstructures with different geometries were introduced into NASICON-type Li1.5Al0.5Ti1.5(PO4)3 oxide solid electrolyte layers via laser ablation. The obtained porous scaffold was infiltrated with various cathode slurries containing cathode active material and an ion-conducting polymer electrolyte to fabricate hybrid composite cathodes with an improved electrode-electrolyte interface. Scanning electron microscopy and energy-dispersive X-ray spectroscopy confirmed a high pore filling degree. A promising specific discharge capacity of 120.1 mAh·g−1 was achieved during electrochemical testing of a prototype all-solid-state battery with a LiNi0.6Mn0.2Co0.2O2 composite cathode and a lithium metal anode. Overall, this work serves as a proof-of-concept for the novel, matrix-supported cell design and provides insights into the production processes involved. |
| 536 | _ | _ | |a 1222 - Components and Cells (POF4-122) |0 G:(DE-HGF)POF4-1222 |c POF4-122 |f POF IV |x 0 |
| 536 | _ | _ | |a ProFeLi - Produktionstechnik für Festkörperbatterien mit Lithium-Metall-Anode (13XP0184B) |0 G:(BMBF)13XP0184B |c 13XP0184B |x 1 |
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| 700 | 1 | _ | |a Zaeh, Michael F. |0 P:(DE-HGF)0 |b 8 |
| 773 | _ | _ | |a 10.1016/j.ensm.2023.03.008 |g Vol. 57, p. 607 - 617 |0 PERI:(DE-600)2841602-8 |p 607 - 617 |t Energy storage materials |v 57 |y 2023 |x 2405-8289 |
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