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| Hauptseite > Publikationsdatenbank > Chitosan as Enabling Polymeric Binder Material for Silicon‐Graphite‐Based Anodes in Lithium‐Ion Batteries > print |
| Hauptseite > Publikationsdatenbank > Chitosan as Enabling Polymeric Binder Material for Silicon‐Graphite‐Based Anodes in Lithium‐Ion Batteries > print |
| 001 | 1024548 | ||
| 005 | 20250203103129.0 | ||
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| 037 | _ | _ | |a FZJ-2024-02228 |
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| 100 | 1 | _ | |a Hamzelui, Niloofar |b 0 |
| 245 | _ | _ | |a Chitosan as Enabling Polymeric Binder Material for Silicon‐Graphite‐Based Anodes in Lithium‐Ion Batteries |
| 260 | _ | _ | |a Weinheim [u.a.] |c 2023 |b Wiley-VCH |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1712737836_24403 |2 PUB:(DE-HGF) |
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| 500 | _ | _ | |a Unterstützt durch Projekt: “GrEEn”(no. 313-W044B) |
| 520 | _ | _ | |a Massive volume change during (de-)lithiation and subsequent challenges, such as pulverization of active materials, delamination of electrode from the current collector, and fragile solid electrolyte interphase, are among the main impediments hindering the large-scale commercialization of silicon-containing anode materials in lithium-ion batteries. In this regard, designer polymeric binders with unique chemistries are considered as enabling solutions. Polymeric materials endowed with functional groups such as –OH, –COOH/COO−, and –NH2/NH3+, capable of building strong H bonds, are hailed as effective binders for Si-containing anode materials. Herein, chitosan biopolymers are investigated as a green and environmentally friendly binder in a silicon/graphite (Si/Gr) anode and compared to lithium poly(acrylic acid)/sodium carboxymethyl cellulose binders. The effect of degree of acetylation (DA) and degree of polymerization of chitosan on the electrochemical performance of Si/Gr anode-based cells is investigated. Anodes with chitosan binder with DA of 50% show the most promising electrochemical performance in Si/Gr||lithium metal and lithium nickel manganese cobalt oxide (NMC622)||Si/Gr cells. Crosslinking of chitosan binder with citric acid monohydrate in combination with free-standing electrodes results in improved electrochemical performance in full cells. The surface chemistry of electrochemically cycled Si/Gr anodes with/without chitosan binder is investigated by X-ray photoelectron spectroscopy. |
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| 700 | 1 | _ | |a Martin Nyenhuis, Gabriela |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Haneke, Lukas |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Eshetu, Gebrekidan Gebresilassie |0 0000-0001-8834-2766 |b 4 |e Corresponding author |
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| 773 | _ | _ | |a 10.1002/ente.202201239 |g Vol. 11, no. 3, p. 2201239 |0 PERI:(DE-600)2700412-0 |n 3 |p 2201239 |t Energy technology |v 11 |y 2023 |x 2194-4288 |
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