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000010251 084__ $$2WoS$$aPhysics, Condensed Matter
000010251 1001_ $$0P:(DE-Juel1)VDB82898$$aWagner, C.$$b0$$uFZJ
000010251 245__ $$aRepulsion between molecules on a metal: Monolayers and submonolayers of hexa-peri-hexabenzocoronene on Au(111)
000010251 260__ $$aCollege Park, Md.$$bAPS$$c2010
000010251 300__ $$a035423
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000010251 440_0 $$04919$$aPhysical Review B$$v81$$x1098-0121$$y3
000010251 500__ $$aFinancial support by Deutsche Forschungsgemeinschaft (DFG) Grants No. FR875/9 and No. FR875/11 is gratefully acknowledged.
000010251 520__ $$aWe investigate the growth of hexa-peri-hexabenzocoronene (HBC) on Au(111) for monolayer (ML) and sub-ML coverage by scanning tunneling microscopy and low-energy electron diffraction. A transition from a disordered isotropic phase at low coverage to a highly ordered phase with a coverage-dependent lattice constant at higher coverage is found and attributed to a repulsive intermolecular force. To deduce the origin of this repulsion a model is set up, containing the Coulomb interaction between molecules and between localized dipoles from the push-back effect, as well as the intermolecular van der Waals potential. The modeling of the van der Waals interaction is done on a force field level. We find that the observed repulsion can only be explained when assuming a certain screening of the attractive London forces by the presence of the metal substrate.
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000010251 7001_ $$0P:(DE-HGF)0$$aKasemann, D.$$b1
000010251 7001_ $$0P:(DE-HGF)0$$aGolnik, C.$$b2
000010251 7001_ $$0P:(DE-HGF)0$$aForker, R.$$b3
000010251 7001_ $$0P:(DE-HGF)0$$aEsselinger, M.$$b4
000010251 7001_ $$0P:(DE-HGF)0$$aMüllen, K.$$b5
000010251 7001_ $$0P:(DE-HGF)0$$aFritz, T.$$b6
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000010251 773__ $$0PERI:(DE-600)2844160-6$$a10.1103/PhysRevB.81.035423$$gVol. 81, p. 035423$$n3$$p035423$$q81<035423$$tPhysical review / B$$v81$$x1098-0121$$y2010
000010251 8567_ $$uhttp://dx.doi.org/10.1103/PhysRevB.81.035423
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