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@ARTICLE{Fu:1025218,
      author       = {Fu, Shuo and Arinicheva, Yulia and Hüter, Claas and
                      Finsterbusch, Martin and Spatschek, Robert},
      title        = {{G}rain {B}oundary {C}haracterization and {P}otential
                      {P}ercolation of the {S}olid {E}lectrolyte {LLZO}},
      journal      = {Batteries},
      volume       = {9},
      number       = {4},
      issn         = {2313-0105},
      address      = {Basel},
      publisher    = {MDPI},
      reportid     = {FZJ-2024-02786},
      pages        = {222 -},
      year         = {2023},
      abstract     = {The influence of different processing routes and grain size
                      distributions on the character of the grain boundaries in
                      Li7La3Zr2O12 (LLZO) and the potential influence on failure
                      through formation of percolating lithium metal networks in
                      the solid electrolyte are investigated. Therefore, high
                      quality hot-pressed Li7La3Zr2O12 pellets are synthesised
                      with two different grain size distributions. Based on the
                      electron backscatter diffraction measurements, the grain
                      boundary network including the grain boundary distribution
                      and its connectivity via triple junctions are analysed
                      concerning potential Li plating along certain susceptible
                      grain boundary clusters in the hot-pressed LLZO pellets.
                      Additionally, the study investigates the possibility to
                      interpret short-circuiting caused by Li metal plating or
                      penetration in all-solid-state batteries through percolation
                      mechanisms in the solid electrolyte microstructure, in
                      analogy to grain boundary failure processes in metallic
                      systems.},
      cin          = {IEK-1 / IEK-2},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-1-20101013 / I:(DE-Juel1)IEK-2-20101013},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / 1222 -
                      Components and Cells (POF4-122) / DFG project 491111487 -
                      Open-Access-Publikationskosten / 2022 - 2024 /
                      Forschungszentrum Jülich (OAPKFZJ) (491111487)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(DE-HGF)POF4-1222 /
                      G:(GEPRIS)491111487},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000980882600001},
      doi          = {10.3390/batteries9040222},
      url          = {https://juser.fz-juelich.de/record/1025218},
}