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001030750 005__ 20240911204733.0
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001030750 1001_ $$0P:(DE-Juel1)130438$$aWilden, Andreas$$b0$$eCorresponding author$$ufzj
001030750 245__ $$aPATRICIA Deliverable D1.4 FP and Am behaviour with new CHON system
001030750 260__ $$c2024
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001030750 520__ $$aA new CHON AmSEL system was developed based on PrOH-BPTD as the americium-selective complexant. Previous investigations (see deliverable D1.1) found it to show sufficient efficiency and selectivity for americium over trivalent lanthanides and curium. PrOH-BPTD is able to complex Am(III) at nominal Am concentrations up to 20 mmol L−1 Am(III), without precipitate of third phase formation. High selectivity is also achieved in the presence of nominal concentrations of Ln(III), although a saturation effect is observed, reducing the selectivity over light lanthanides (especially La(III)). The resistance to alpha radiolysis was found to be excellent. The non-lanthanide fission products Mo, Sr, Zr, and Pd could potentially be co-stripped with Am, but can be handled using masking agents and nitric acid scrubbing. Only Tc was found to likely follow Am, if present in the PUREX raffinate.
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001030750 7001_ $$0P:(DE-Juel1)167486$$aSauerwein, Fynn Sören$$b1$$ufzj
001030750 7001_ $$0P:(DE-Juel1)164342$$aSchneider, Dimitri$$b2$$ufzj
001030750 7001_ $$0P:(DE-Juel1)130395$$aPaparigas, Zaina$$b3$$ufzj
001030750 7001_ $$0P:(DE-Juel1)176390$$aHenkes, Maximilian$$b4$$ufzj
001030750 7001_ $$0P:(DE-Juel1)130383$$aModolo, Giuseppe$$b5$$ufzj
001030750 7001_ $$0P:(DE-HGF)0$$aBaruth, Giana$$b6
001030750 7001_ $$0P:(DE-HGF)0$$aWeßling, Patrik$$b7
001030750 7001_ $$0P:(DE-HGF)0$$aGeist, Andreas$$b8
001030750 7001_ $$0P:(DE-HGF)0$$aMarie, Cecile$$b9
001030750 7001_ $$0P:(DE-HGF)0$$aGracia, Sophie$$b10
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