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| Home > Publications database > PATRICIA Deliverable D1.4 FP and Am behaviour with new CHON system > print |
| 001 | 1030750 | ||
| 005 | 20240911204733.0 | ||
| 037 | _ | _ | |a FZJ-2024-05453 |
| 041 | _ | _ | |a English |
| 100 | 1 | _ | |a Wilden, Andreas |0 P:(DE-Juel1)130438 |b 0 |e Corresponding author |u fzj |
| 245 | _ | _ | |a PATRICIA Deliverable D1.4 FP and Am behaviour with new CHON system |
| 260 | _ | _ | |c 2024 |
| 300 | _ | _ | |a 15 p. |
| 336 | 7 | _ | |a report |2 DRIVER |
| 336 | 7 | _ | |a REPORT |2 ORCID |
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| 336 | 7 | _ | |a TECHREPORT |2 BibTeX |
| 336 | 7 | _ | |a Internal Report |b intrep |m intrep |0 PUB:(DE-HGF)15 |s 1726029985_22745 |2 PUB:(DE-HGF) |
| 520 | _ | _ | |a A new CHON AmSEL system was developed based on PrOH-BPTD as the americium-selective complexant. Previous investigations (see deliverable D1.1) found it to show sufficient efficiency and selectivity for americium over trivalent lanthanides and curium. PrOH-BPTD is able to complex Am(III) at nominal Am concentrations up to 20 mmol L−1 Am(III), without precipitate of third phase formation. High selectivity is also achieved in the presence of nominal concentrations of Ln(III), although a saturation effect is observed, reducing the selectivity over light lanthanides (especially La(III)). The resistance to alpha radiolysis was found to be excellent. The non-lanthanide fission products Mo, Sr, Zr, and Pd could potentially be co-stripped with Am, but can be handled using masking agents and nitric acid scrubbing. Only Tc was found to likely follow Am, if present in the PUREX raffinate. |
| 536 | _ | _ | |a 1412 - Predisposal (POF4-141) |0 G:(DE-HGF)POF4-1412 |c POF4-141 |f POF IV |x 0 |
| 536 | _ | _ | |a PATRICIA - Partitioning And Transmuter Research Initiative in a Collaborative Innovation Action (945077) |0 G:(EU-Grant)945077 |c 945077 |f NFRP-2019-2020 |x 1 |
| 588 | _ | _ | |a Dataset connected to DataCite |
| 700 | 1 | _ | |a Sauerwein, Fynn Sören |0 P:(DE-Juel1)167486 |b 1 |u fzj |
| 700 | 1 | _ | |a Schneider, Dimitri |0 P:(DE-Juel1)164342 |b 2 |u fzj |
| 700 | 1 | _ | |a Paparigas, Zaina |0 P:(DE-Juel1)130395 |b 3 |u fzj |
| 700 | 1 | _ | |a Henkes, Maximilian |0 P:(DE-Juel1)176390 |b 4 |u fzj |
| 700 | 1 | _ | |a Modolo, Giuseppe |0 P:(DE-Juel1)130383 |b 5 |u fzj |
| 700 | 1 | _ | |a Baruth, Giana |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Weßling, Patrik |0 P:(DE-HGF)0 |b 7 |
| 700 | 1 | _ | |a Geist, Andreas |0 P:(DE-HGF)0 |b 8 |
| 700 | 1 | _ | |a Marie, Cecile |0 P:(DE-HGF)0 |b 9 |
| 700 | 1 | _ | |a Gracia, Sophie |0 P:(DE-HGF)0 |b 10 |
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| 913 | 1 | _ | |a DE-HGF |b Forschungsbereich Energie |l Nukleare Entsorgung, Sicherheit und Strahlenforschung (NUSAFE II) |1 G:(DE-HGF)POF4-140 |0 G:(DE-HGF)POF4-141 |3 G:(DE-HGF)POF4 |2 G:(DE-HGF)POF4-100 |4 G:(DE-HGF)POF |v Nukleare Entsorgung |9 G:(DE-HGF)POF4-1412 |x 0 |
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| 980 | _ | _ | |a UNRESTRICTED |
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