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@ARTICLE{Jugovac:1048406,
author = {Jugovac, M. and Cojocariu, I. and Bihlmayer, Gustav and
Gargiani, P. and Valvidares, M. and Brondin, C. A. and
Blügel, Stefan and Locatelli, A. and Mentes, T. O. and
Perna, P.},
title = {{P}ersistent {M}agnetism and {T}unable {D}oping of
{M}onolayer {G}raphene via {E}uropium {D}ensity
{M}odulation},
journal = {Advanced science},
volume = {},
issn = {2198-3844},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2025-04618},
pages = {e21592},
year = {2025},
abstract = {Reaching the van Hove singularity (VHS) in a material
enables the emergence of exotic electronic and magnetic
phases, such as superconductivity and the quantum anomalous
Hall effect. This is demonstrated in cuprates,magic-angle
bilayer graphene, and more recently, monolayer graphene
interfaced with alkali and rare earth elements. Here, the
europium density at the graphene/rhenium interface is
modulated to tune the electron doping level in monolayer
graphene across the VHS point, forming either a dense or
diluted europium phase. The dense phase enables flat bands
at the Fermi level, while graphene remains decoupled from
the Re(0001) substrate in both cases. The Dirac point is
shifted over 1.5 eV below the Fermi level, and europium
lifts the degeneracy of the Dirac cones: one branch
hybridizes with Eu 4f states, the other retains Dirac-like
dispersion, as corroborated by density functional theory.
X-ray absorption spectroscopy reveals a mixed Eu(II)/Eu(III)
valence state in the dense phase and the persistence of Eu
magnetic response up to room temperature in both. The
intercalated phases exhibit exceptional thermal stability,
with the diluted phase stable up to 960 K. These results
highlight the potential of rare-earth-doped graphene for
engineering flat bands, tunable Dirac-cone splitting, and
robust interfacial magnetism.},
cin = {PGI-1 / JARA-HPC},
ddc = {624},
cid = {I:(DE-Juel1)PGI-1-20110106 / $I:(DE-82)080012_20140620$},
pnm = {5211 - Topological Matter (POF4-521) / SFB 1238 C01 -
Strukturinversionsasymmetrische Materie und
Spin-Orbit-Phänomene mittels ab initio (C01) (319898210)},
pid = {G:(DE-HGF)POF4-5211 / G:(GEPRIS)319898210},
typ = {PUB:(DE-HGF)16},
doi = {10.1002/advs.202521592},
url = {https://juser.fz-juelich.de/record/1048406},
}