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@INPROCEEDINGS{Wolf:1051653,
author = {Wolf, Niklas and Javed, Ali and Treutlein, Leander and
Kungl, Hans and Jodat, Eva and Karl, André and Eichel,
Rüdiger-A.},
title = {{I}mpact of {M}embrane {E}lectrode {A}ssembly
{C}onditioning on the {P}erformance of {P}roton {E}xchange
{M}embrane {E}lectrolytic {C}ells: {I}nsights into
{S}hort-{T}erm and {L}ong-{T}erm {O}peration},
issn = {2151-2043},
reportid = {FZJ-2026-00562},
year = {2025},
abstract = {Proton Exchange Membrane Electrolysis is a promising
technology for efficient hydrogen production, utilizing the
electrolysis of water to generate hydrogen. The performance
of Proton Exchange Membrane Electrolytic Cells (PEMECs) is
strongly influenced by the conditioning of the Membrane
Electrode Assembly (MEA), which serves as a critical step in
preparing the MEA for optimal functionality. The
conditioning process includes two steps. The pre-treatment,
which involves hydrating and chemically or thermally
activating the MEA, followed by a break-in procedure that
stabilizes the electrochemical performance during initial
operation.The conditioning strategies explored in this study
include ex-situ and in-situ hydration, acidic treatment, and
elevated temperature conditions during the pre-treatment
step. The impact of pre-treatment conditions; mechanical,
chemical, and thermal on the short-term electrochemical
performance of Nafion™ N115-based MEAs highlight the
importance of both the pre-treatment and break-in procedures
in establishing consistent cell operation.The results show
that in-situ pre-treatment allows the membrane to swell
under constrained conditions post-assembly, significantly
enhances the contact area between the MEA and the porous
transport layers, reducing contact resistance and improving
overall PEMEC performance. Moreover, acidic treatment and
elevated temperature conditions further contribute to
improved proton conductivity, leading to reduced Ohmic
resistance and cell voltage.While the break-in procedure
stabilizes the cell’s electrochemical performance in the
short term, further investigation is conducted to evaluate
how these conditioning protocols impact the long-term
degradation mechanisms. This study presents preliminary
findings on the durability of conditioned MEAs under
continuous operation and explores how optimizing the
conditioning process could contribute to enhanced long-term
performance, paving the way for more reliable and efficient
PEMEC systems in industrial applications.},
month = {May},
date = {2025-05-18},
organization = {247th ECS Meeting, Montreal, Québec
(Kanada), 18 May 2025 - 22 May 2025},
subtyp = {Other},
cin = {IET-1},
ddc = {540},
cid = {I:(DE-Juel1)IET-1-20110218},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123) / HITEC -
Helmholtz Interdisciplinary Doctoral Training in Energy and
Climate Research (HITEC) (HITEC-20170406)},
pid = {G:(DE-HGF)POF4-1231 / G:(DE-Juel1)HITEC-20170406},
typ = {PUB:(DE-HGF)6},
doi = {10.1149/MA2025-01381941mtgabs},
url = {https://juser.fz-juelich.de/record/1051653},
}