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| Hauptseite > Publikationsdatenbank > Neutron diffraction investigation of the crystal and magnetic structures in KCrF3 perovskite > print |
| Hauptseite > Publikationsdatenbank > Neutron diffraction investigation of the crystal and magnetic structures in KCrF3 perovskite > print |
| 001 | 11329 | ||
| 005 | 20250129094219.0 | ||
| 024 | 7 | _ | |a 10.1103/PhysRevB.82.094437 |2 DOI |
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| 082 | _ | _ | |a 530 |
| 084 | _ | _ | |2 WoS |a Physics, Condensed Matter |
| 100 | 1 | _ | |0 P:(DE-Juel1)131047 |a Xiao, Y. |b 0 |u FZJ |
| 245 | _ | _ | |a Neutron diffraction investigation of the crystal and magnetic structures in KCrF3 perovskite |
| 260 | _ | _ | |a College Park, Md. |b APS |c 2010 |
| 300 | _ | _ | |a 094437 |
| 336 | 7 | _ | |a Journal Article |0 PUB:(DE-HGF)16 |2 PUB:(DE-HGF) |
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| 440 | _ | 0 | |0 4919 |a Physical Review B |v 82 |x 1098-0121 |y 9 |
| 500 | _ | _ | |a Record converted from VDB: 12.11.2012 |
| 520 | _ | _ | |a KCrF3 represents another prototypical orbital-ordered perovskite, where Cr2+ possesses the same electronic configuration of 3d(4) as that of strongly Jahn-Teller distorted Mn3+ in many colossal magnetoresistance manganites. The crystal and magnetic structures of KCrF3 compound are investigated by using polarized and unpolarized neutron powder-diffraction methods. The results show that the KCrF3 compound crystallizes in tetragonal structure at room temperature and undergoes a monoclinic distortion with the decrease in temperature. The distortion of the crystal structure indicates the presence of cooperative Jahn-Teller distortion which is driven by orbital ordering. With decreasing temperature, four magnetic phase transitions are observed at 79.5, 45.8, 9.5, and 3.2 K, which suggests a rich magnetic phase diagram. Below T-N = 79.5 K, the Cr2+ moment orders in an incommensurate antiferromagnetic arrangement, which can be defined by the magnetic propagation vector (1/2 + delta, 1/2 + delta, 0). The incommensurate-commensurate magnetic transition occurs at 45.8 K and the magnetic propagation vector locks into (1/2, 1/2, 0) with the Cr moment of 3.34(5) mu(B), aligned ferromagnetically in (220) plane, but antiferromagnetically along [110] direction. Below 9.5 K, the canted antiferromagnetic ordering and weak ferromagnetism arise from the collinear antiferromagnetic structure while the Dzyaloshinskii-Moriya interaction and tilted character of the single-ion anisotropy might give rise to the complex magnetic behaviors below 9.5 K. |
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| 700 | 1 | _ | |0 P:(DE-Juel1)VDB84209 |a Kumar, C. M. N. |b 3 |u FZJ |
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