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@BOOK{Urban:12159,
author = {Urban, Susanna},
title = {{C}harakterisierung der {Q}uellverteilung von {F}einstaub
und {S}tickoxiden in ländlichem und städtischem {G}ebiet},
volume = {84},
issn = {1866-1793},
school = {Universität Wuppertal},
type = {Dr.},
address = {Jülich},
publisher = {Forschungszentrum Jülich GmbH Zentralbibliothek, Verlag},
reportid = {PreJuSER-12159},
isbn = {978-3-89336-669-9},
series = {Schriften des Forschungszentrums Jülich : Energie $\&$
Umwelt / Energy $\&$ Environment},
pages = {VI, 211 S.},
year = {2010},
note = {Record converted from JUWEL: 18.07.2013; Univ. Wuppertal,
Diss., 2010},
abstract = {By the entry of anthropogenic emissions, the air quality is
especially impacted in urban center. Thus, EU-wide limits of
gas phase components, e.g. NO$_{2}$ und O$_{3}$, and
particulate matter concentration (PM10) exist to protect
human health. Particulary, high particulate matter
concentrations are more and more of interest because of
their adverse health effect on the human respiratory system.
Therefore a network of stationary measurements in different
loaded and inhabited regions monitors the air quality in
Germany. In contrast to these selective stationary
facilities, this thesis presents mobile measurements to
determine concentration fields of gases and particles.
Therefore, a ”driving air-lab“ with a large set of
temporally high resolved instruments to measure gas and
particulate phase as well as geographical and meteorological
parameters has been built up. The particulate measurement
technique includes PM10- and PM2.5-collections and real-time
ELPI measurements of time resolved particle size
concentrations. Additionally, the installation of gas phase
detection technique for NO$_{2}$, NO, O$_{3}$, CO as well as
for volatile organic hydrocarbons completes the ” driving
air-lab“. During the three measurement campaigns lasting
several weeks the temporal and spatial distribution of
particulate and gas phase concentrations in rural, suburban
and urban area in the region of the Bodensee, in the city
region of Düsseldorf and close to the highway in the area
of Jülich could be determined and classified. During the
measurement campaign ZEPTER-2 the ” driving air-lab“
formed the groundbase to the concurrent vertical profile
measurements of the zeppelin. The comparison of the
measuring systems of all parameters during the intermediate
landing of the zeppelin showed a very good agreement. The
use of adequate percentile filters allowed the separation of
the local traffic peaks from the total background. It could
be demonstrated that the total background is composed of
quantifying fractions of the regional and the urban
background. The difference of the current measuring signals
and the regional background represents the maximum
achievable release potential through traffic related
activities for traffic dominated trace substances. Moreover,
typical particulate size distributions and VOC-compositions
of different contamination scenarios (urban, suburban and
rural with biogenic contribution) could be determined.
Adequate weather conditions approved the investigation of
inversion layers of trace substances by the passing of a
mountain when using the ” driving air-lab“. During the
measurement campaign in Düsseldorf three characteristic
measuring scenarios of a city, arterial streets, side
streets and a tunnel, were distinguished. The correlation
analysis showed a coemission of particles and nitrogen
oxides. Furthermore, a total background concentration-field
with street resolution of a residential area was created
which reveals that the representativeness of a hypothetical
measuring station only reaches a few 100 m. The
multiregression analysis with source pattern of different
engine systems in variable operating conditions demonstrated
that the main contribution of the VOC-emissions derives from
gasoline engines in cold start status.},
cin = {IEK-8},
ddc = {500},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK406},
typ = {PUB:(DE-HGF)3},
url = {https://juser.fz-juelich.de/record/12159},
}