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@ARTICLE{Wellert:15317,
author = {Wellert, S. and Tiersch, B. and Koetz, J. and Richardt, A.
and Lapp, A. and Holderer, O. and Gäb, J. and Blum, M.-M.
and Schulreich, C. and Stehle, R. and Hellweg, T.},
title = {{T}he {DFP}ase from {L}oligo vulgaris in sugar
surfactant-based bicontinuous microemulsions: structure,
dynamics, and enzyme activity},
journal = {European biophysics journal},
volume = {40},
issn = {0175-7571},
address = {Berlin},
publisher = {Springer},
reportid = {PreJuSER-15317},
pages = {761 - 774},
year = {2011},
note = {J.G. and M.M.B. were supported by the German Ministry of
Defense under contract E/UR3G/6G115/6A801. T. H., R. S., C.
S. also were financed by the German Ministry of Defense
(Contracts E/E590/9Z004/5F159 and E/E590/8Z002/4F170). The
SANS experiments were supported by the European Union
through the NMI3 program. We are grateful to the Laboratoire
Leon Brillouin and the Julich Center for Neutron Scattering
at the FRM II for providing beamtime.},
abstract = {The enzyme diisopropyl fluorophosphatase (DFPase) from the
squid Loligo vulgaris is of great interest because of its
ability to catalyze the hydrolysis of highly toxic
organophosphates. In this work, the enzyme structure in
solution (native state) was studied by use of different
scattering methods. The results are compared with those from
hydrodynamic model calculations based on the DFPase crystal
structure. Bicontinuous microemulsions made of sugar
surfactants are discussed as host systems for the DFPase.
The microemulsion remains stable in the presence of the
enzyme, which is shown by means of scattering experiments.
Moreover, activity assays reveal that the DFPase still has
high activity in this complex reaction medium. To complement
the scattering experiments cryo-SEM was also employed to
study the microemulsion structure.},
keywords = {Animals / Carbohydrates: chemistry / Carbohydrates:
pharmacology / Emulsions / Loligo: enzymology / Loligo:
metabolism / Microscopy, Electron, Scanning / Neutron
Diffraction / Phosphoric Triester Hydrolases: analysis /
Phosphoric Triester Hydrolases: chemistry / Phosphoric
Triester Hydrolases: metabolism / Scattering, Small Angle /
Solutions: chemistry / Surface-Active Agents: chemistry /
Surface-Active Agents: pharmacology / Carbohydrates (NLM
Chemicals) / Emulsions (NLM Chemicals) / Solutions (NLM
Chemicals) / Surface-Active Agents (NLM Chemicals) /
Phosphoric Triester Hydrolases (NLM Chemicals) /
diisopropyl-fluorophosphatase (NLM Chemicals) / J (WoSType)},
cin = {ICS-1 / JCNS (München) ; Jülich Centre for Neutron
Science JCNS (München) ; JCNS-FRM-II / JCNS-1},
ddc = {570},
cid = {I:(DE-Juel1)ICS-1-20110106 /
I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106},
pnm = {BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung / Großgeräte für die Forschung
mit Photonen, Neutronen und Ionen (PNI)},
pid = {G:(DE-Juel1)FUEK505 / G:(DE-Juel1)FUEK415},
experiment = {EXP:(DE-MLZ)J-NSE-20140101},
shelfmark = {Biophysics},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:21416312},
UT = {WOS:000290331400006},
doi = {10.1007/s00249-011-0689-0},
url = {https://juser.fz-juelich.de/record/15317},
}