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@ARTICLE{Mulder:155433,
      author       = {Mulder, M. D. and Heil, A. and Kukučka, P. and Klánová,
                      J. and Kuta, J. and Prokeš, R. and Sprovieri, F. and
                      Lammel, G.},
      title        = {{P}olycyclic aromatic hydrocarbons in atmospheric aerosols
                      and air–sea exchange in the {M}editerranean},
      journal      = {Atmospheric chemistry and physics / Discussions},
      volume       = {14},
      number       = {5},
      issn         = {1680-7375},
      address      = {Katlenburg-Lindau},
      publisher    = {EGU},
      reportid     = {FZJ-2014-04599},
      pages        = {5963 - 5990},
      year         = {2014},
      abstract     = {Polycyclic aromatic hydrocarbons (PAH) concentration in air
                      of the central and eastern Mediterranean in summer 2010 was
                      1.45 (0.30–3.25) ng m−3, with $≈8\%$ in the
                      particulate phase, associated with particles < 0.25 μm. The
                      diffusive air–sea exchange fluxes of fluoranthene and
                      pyrene were mostly found net-depositional or close to phase
                      equilibrium, while retene was net-volatilisational in a
                      large sea region. Regional fire activity records in
                      combination with box model simulations suggest that seasonal
                      depositional input of retene from biomass burning into the
                      surface waters during summer is followed by an annual
                      reversal of air–sea exchange, while inter-annual
                      variability is dominated by the variability of the fire
                      season. It is concluded that future negative emission trends
                      or interannual variability of regional sources may trigger
                      the sea to become a secondary PAH source through reversal of
                      diffusive air–sea exchange.},
      cin          = {IEK-8},
      ddc          = {550},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {233 - Trace gas and aerosol processes in the troposphere
                      (POF2-233)},
      pid          = {G:(DE-HGF)POF2-233},
      typ          = {PUB:(DE-HGF)16},
      doi          = {10.5194/acpd-14-5963-2014},
      url          = {https://juser.fz-juelich.de/record/155433},
}