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@ARTICLE{Becker:201007,
author = {Becker, J. Sabine and Matusch, Andreas and Wu, Bei},
title = {{B}ioimaging mass spectrometry of trace elements – recent
advance and applications of {LA}-{ICP}-{MS}: {A} review},
journal = {Analytica chimica acta},
volume = {835},
issn = {0003-2670},
address = {Amsterdam},
publisher = {Elsevier Science},
reportid = {FZJ-2015-03321},
pages = {1 - 18},
year = {2014},
abstract = {Bioimaging using laser ablation inductively coupled plasma
mass spectrometry (LA-ICP-MS) offers the capability to
quantify trace elements and isotopes within tissue sections
with a spatial resolution ranging about 10–100 μm.
Distribution analysis adds to clarifying basic questions of
biomedical research and enables bioaccumulation and
bioavailability studies for ecological and toxicological
risk assessment in humans, animals and plants. Major
application fields of mass spectrometry imaging (MSI) and
metallomics have been in brain and cancer research, animal
model validation, drug development and plant science. Here
we give an overview of latest achievements in methods and
applications. Recent improvements in ablation systems,
operation and cell design enabled progressively better
spatial resolutions down to 1 μm. Meanwhile, a body of
research has accumulated covering basic principles of the
element architecture in animals and plants that could
consistently be reproduced by several laboratories such as
the distribution of Fe, Cu, Zn in rodent brain. Several
studies investigated the distribution and delivery of
metallo-drugs in animals. Hyper-accumulating plants and
pollution indicator organisms have been the key topics in
environmental science. Increasingly, larger series of
samples are analyzed, may it be in the frame of comparisons
between intervention and control groups, of time kinetics or
of three-dimensional atlas approaches.},
cin = {ZEA-3 / INM-2},
ddc = {540},
cid = {I:(DE-Juel1)ZEA-3-20090406 / I:(DE-Juel1)INM-2-20090406},
pnm = {313 - Cancer risk factors and prevention (POF2-313)},
pid = {G:(DE-HGF)POF2-313},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000338713400001},
doi = {10.1016/j.aca.2014.04.048},
url = {https://juser.fz-juelich.de/record/201007},
}