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@ARTICLE{Dutta:201160,
author = {Dutta, Suryendu and Hartkopf-Fröder, Christoph and Witte,
Karin and Brocke, Rainer and Mann, Ulrich},
title = {{M}olecular characterization of fossil palynomorphs by
transmission micro-{FTIR} spectroscopy: {I}mplications for
hydrocarbon source evaluation},
journal = {International journal of coal geology},
volume = {115},
issn = {0166-5162},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2015-03465},
pages = {13 - 23},
year = {2013},
abstract = {Transmission micro-FTIR spectroscopy has been conducted to
elucidate the macromolecular structure of well-preserved
fossil palynomorphs including prasinophycean algae,
megaspores, chitinozoans, and scolecodonts. Plant and
arthropod cuticles which may be present in palynological
residues have also been investigated. Important differences
are noted among these palynomorph groups regarding the
intensities of CHx, Cdouble bond; length as m-dashO and
aromatic Cdouble bond; length as m-dashC absorptions.
Tasmanites, Leiosphaeridia, and plant cuticles are
characterized by stronger aliphatic CHx stretching
(3000–2800 cm− 1), strong CH3 (1460–1450 cm− 1), and
intense Cdouble bond; length as m-dashO group (1710–1700
cm− 1) absorptions. Aromatic Cdouble bond; length as
m-dashC stretching (1610–1560 cm− 1) absorptions are
less intense and aromatic CH out of plane (900–750 cm−
1) absorptions are absent. In contrast, chitinozoans,
scolecodonts, and arthropod cuticles show intense aromatic
Cdouble bond; length as m-dashC stretching (1620–1560
cm− 1) and aromatic CH out of plane (900–750 cm− 1)
absorptions. Aliphatic CHx stretching (3000–2800 cm− 1)
and Cdouble bond; length as m-dashO group (1710–1700 cm−
1) absorptions are less intense. Megaspores are
characterized by stronger aliphatic CHx stretching
(3000–2800 cm− 1), strong CH3 (1460–1450 cm− 1), and
moderate aromatic Cdouble bond; length as m-dashC stretching
(1610–1560 cm− 1) and Cdouble bond; length as m-dashO
group (1710–1700 cm− 1) absorptions. The CH2/CH3
intensity ratio has been used to assess the relative chain
length and degree of branching. The aliphatic components in
Tasmanites, Leiosphaeridia, and plant cuticles are longest
chained and least branched whereas those in chitinozoans,
scolecodonts, and arthropod cuticles are shortest chained
and most branched. Megaspores show intermediate CH2/CH3
ratio. The present study demonstrates that palynomorphs
differ in functional group chemistry and this spectroscopic
technique can be useful to assign biological affinity of
enigmatic palynomorphs. Furthermore, micro-FTIR spectroscopy
provides insights into the hydrocarbon generating potential
of different fossil palynomorph groups.},
cin = {IBG-3},
ddc = {550},
cid = {I:(DE-Juel1)IBG-3-20101118},
pnm = {246 - Modelling and Monitoring Terrestrial Systems: Methods
and Technologies (POF2-246) / 255 - Terrestrial Systems:
From Observation to Prediction (POF3-255)},
pid = {G:(DE-HGF)POF2-246 / G:(DE-HGF)POF3-255},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000322611100002},
doi = {10.1016/j.coal.2013.04.003},
url = {https://juser.fz-juelich.de/record/201160},
}