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@ARTICLE{Chiesa:201445,
author = {Chiesa, Alessandro and Whitehead, George F. S. and
Carretta, Stefano and Carthy, Laura and Timco, Grigore A.
and Teat, Simon J. and Amoretti, Giuseppe and Pavarini, Eva
and Winpenny, Richard E. P. and Santini, Paolo},
title = {{M}olecular nanomagnets with switchable coupling for
quantum simulation},
journal = {Scientific reports},
volume = {4},
issn = {2045-2322},
address = {London},
publisher = {Nature Publishing Group},
reportid = {FZJ-2015-03740},
pages = {7423 -},
year = {2014},
abstract = {Molecular nanomagnets are attractive candidate qubits
because of their wide inter- and intra-molecular tunability.
Uniform magnetic pulses could be exploited to implement one-
and two-qubit gates in presence of a properly engineered
pattern of interactions, but the synthesis of suitable and
potentially scalable supramolecular complexes has proven a
very hard task. Indeed, no quantum algorithms have ever been
implemented, not even a proof-of-principle two-qubit gate.
Here we show that the magnetic couplings in two
supramolecular {Cr7Ni}-Ni-{Cr7Ni} assemblies can be
chemically engineered to fit the above requisites for
conditional gates with no need of local control. Microscopic
parameters are determined by a recently developed many-body
ab-initio approach and used to simulate quantum gates. We
find that these systems are optimal for proof-of-principle
two-qubit experiments and can be exploited as building
blocks of scalable architectures for quantum simulation.},
cin = {IAS-3},
ddc = {000},
cid = {I:(DE-Juel1)IAS-3-20090406},
pnm = {424 - Exploratory materials and phenomena (POF2-424)},
pid = {G:(DE-HGF)POF2-424},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000346288300001},
pubmed = {pmid:25502419},
doi = {10.1038/srep07423},
url = {https://juser.fz-juelich.de/record/201445},
}