Journal Article FZJ-2015-03740

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Molecular nanomagnets with switchable coupling for quantum simulation

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2014
Nature Publishing Group London

Scientific reports 4, 7423 - () [10.1038/srep07423]

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Abstract: Molecular nanomagnets are attractive candidate qubits because of their wide inter- and intra-molecular tunability. Uniform magnetic pulses could be exploited to implement one- and two-qubit gates in presence of a properly engineered pattern of interactions, but the synthesis of suitable and potentially scalable supramolecular complexes has proven a very hard task. Indeed, no quantum algorithms have ever been implemented, not even a proof-of-principle two-qubit gate. Here we show that the magnetic couplings in two supramolecular {Cr7Ni}-Ni-{Cr7Ni} assemblies can be chemically engineered to fit the above requisites for conditional gates with no need of local control. Microscopic parameters are determined by a recently developed many-body ab-initio approach and used to simulate quantum gates. We find that these systems are optimal for proof-of-principle two-qubit experiments and can be exploited as building blocks of scalable architectures for quantum simulation.

Classification:

Contributing Institute(s):
  1. Theoretische Nanoelektronik (IAS-3)
Research Program(s):
  1. 424 - Exploratory materials and phenomena (POF2-424) (POF2-424)

Appears in the scientific report 2015
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 Record created 2015-06-09, last modified 2024-06-25