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@ARTICLE{Shirpour:201772,
author = {Shirpour, M. and Gregori, G. and Houben, L. and Merkle, R.
and Maier, J.},
title = {{H}igh spatially resolved cation concentration profile at
the grain boundaries of {S}c-doped {B}a{Z}r{O}$_{3}$},
journal = {Solid state ionics},
volume = {262},
issn = {0167-2738},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2015-04066},
pages = {860 - 864},
year = {2014},
abstract = {Recent studies have demonstrated that a higher dopant
concentration in the grain boundary region (which includes
boundary core and neighboring layers) of acceptor-doped
oxides results in a remarkable decrease of grain boundary
electrical resistance. In the present work, the spatial
distribution of cations in the proton conducting scandium
doped barium zirconate is investigated by transmission
electron microscopy with high lateral resolution. Cation
profiles with a resolution of 0.5 nm obtained using electron
energy-loss spectroscopy indicate segregation of a
noticeable part of scandium into the grain boundary core.
This direct observation is consistent with the measured
grain boundary electrical behavior and is interpreted in
terms of the space charge model.},
cin = {PGI-5},
ddc = {530},
cid = {I:(DE-Juel1)PGI-5-20110106},
pnm = {42G - Peter Grünberg-Centre (PG-C) (POF2-42G41)},
pid = {G:(DE-HGF)POF2-42G41},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000338810500187},
doi = {10.1016/j.ssi.2013.11.032},
url = {https://juser.fz-juelich.de/record/201772},
}