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001     202798
005     20210129220231.0
024 7 _ |a 10.1038/ncomms8716
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024 7 _ |a 2128/8986
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100 1 _ |a Mairoser, Thomas
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245 _ _ |a High-quality EuO thin films the easy way via topotactic transformation
260 _ _ |a London
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520 _ _ |a Epitaxy is widely employed to create highly oriented crystalline films. A less appreciated, butnonetheless powerful means of creating such films is via topotactic transformation, in which achemical reaction transforms a single crystal of one phase into a single crystal of a differentphase, which inherits its orientation from the original crystal. Topotactic reactions may beapplied to epitactic films to substitute, add or remove ions to yield epitactic films of differentphases. Here we exploit a topotactic reduction reaction to provide a non-ultra-high vacuum(UHV) means of growing highly oriented single crystalline thin films of the easily overoxidizedhalf-metallic semiconductor europium monoxide (EuO) with a perfection rivallingthat of the best films of the same material grown by molecular-beam epitaxy or UHV pulsedlaserdeposition. As the technique only requires high-vacuum deposition equipment, it hasthe potential to drastically improve the accessibility of high-quality single crystalline films ofEuO as well as other difficult-to-synthesize compounds.
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700 1 _ |a Mundy, Julia A.
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700 1 _ |a Melville, Alexander
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700 1 _ |a Hodash, Daniel
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700 1 _ |a Cueva, Paul
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700 1 _ |a Held, Rainer
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700 1 _ |a Glavic, Artur
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700 1 _ |a Schubert, Jürgen
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700 1 _ |a Muller, David A.
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700 1 _ |a Schlom, Darrell G.
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700 1 _ |a Schmehl, Andreas
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773 _ _ |a 10.1038/ncomms8716
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