Home > Publications database > Water Oxidation Catalyzed by a New Tetracobalt-Substituted Polyoxometalate Complex: [{Co4(µ-OH)(H2O)3}(Si2W19O70)]11 > print

001     22364
005     20190625111242.0
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|a pmid:22186630
024 7 _ |2 DOI
|a 10.1039/C1DT11211B
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041 _ _ |a eng
082 _ _ |a 540
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|a Chemistry, Inorganic & Nuclear
100 1 _ |0 P:(DE-HGF)0
|a Zhu, G.
|b 0
245 _ _ |a Water Oxidation Catalyzed by a New Tetracobalt-Substituted Polyoxometalate Complex: [{Co4(µ-OH)(H2O)3}(Si2W19O70)]11
260 _ _ |a London
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|c 2012
300 _ _ |a 2084 - 2090
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|a Dalton Transactions
|v 41
|x 1477-9226
|y 7
500 _ _ |3 POF3_Assignment on 2016-02-29
500 _ _ |a The present research is supported by grant DE-FG02-03ER15461 from the U.S. Department of Energy. The authors gratefully acknowledge NSF MRI-R2 grant (CHE-0958205) and the use of the resources of the Cherry Emerson Center for Scientific Computation.
520 _ _ |a A new polyoxometalate of earth adundant elements [{Co(4)(μ-OH)(H(2)O)(3)}(Si(2)W(19)O(70))](11-) has been synthesized, characterized and shown to be a water oxidation catalyst. The initial catalytic complex is unstable and slowly undergoes hydrolysis. The hydrolysis products have been isolated and characterized, and their catalytic water oxidation activity is assessed.
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|a Schilder, H.
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|a Song, J.
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|a Zhao, C.
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856 7 _ |u http://dx.doi.org/10.1039/C1DT11211B
856 4 _ |u https://juser.fz-juelich.de/record/22364/files/FZJ-22364.pdf
|y Published under German "Allianz" Licensing conditions on 2011-12-21. Available in OpenAccess from 2012-12-21
|z Published final document.
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