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@ARTICLE{Yu:255767,
      author       = {Yu, Na and Klepov, Vladislav and Neumeier, Stefan and
                      Depmeier, Wulf and Bosbach, Dirk and Suleimanov, Evgeny V.
                      and Alekseev, Evgeny},
      title        = {{F}urther {I}nsight into {U}ranium and {T}horium
                      {M}etaphosphate {C}hemistry and the {E}ffect of {N}d$ ^{3+}$
                      {I}ncorporation into {U}ranium({IV}) {M}etaphosphate},
      journal      = {European journal of inorganic chemistry},
      volume       = {2015},
      number       = {9},
      issn         = {1434-1948},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2015-05881},
      pages        = {1562 - 1568},
      year         = {2015},
      abstract     = {A tetragonal modification of uranium polymetaphosphate
                      U(PO3)4, a mixed U4+/Nd3+ polymetaphosphate
                      “(U0.62Nd0.38)(PO3)4”, and two new tetraphosphates,
                      Th(P4O12) and U(P4O12), were synthesized. The structures of
                      the obtained materials were characterized by X-ray
                      diffraction and Raman spectroscopy. The presence of Nd in
                      (U0.62Nd0.38)(PO3)4 was proven by energy-dispersive X-ray
                      spectroscopy (EDX), and the measured degree of substitution
                      for U agrees well with the X-ray crystallography results;
                      however, the mechanism of the necessary charge compensation
                      could not be identified. The cation arrangements in the
                      crystal structures of thorium and uranium polymetaphosphates
                      have been studied in terms of Voronoi–Dirichlet polyhedra.
                      Different conformations of the tetraphosphate polyanions
                      were observed in the crystal structures of Th(P4O12) and
                      U(P4O12). The Raman spectrum of a single crystal of
                      Th(P4O12) was recorded, and the bands were assigned.},
      cin          = {IEK-6},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-6-20101013},
      pnm          = {161 - Nuclear Waste Management (POF3-161) / Helmholtz Young
                      Investigators Group: Energy (HGF-YIG-Energy) / HITEC -
                      Helmholtz Interdisciplinary Doctoral Training in Energy and
                      Climate Research (HITEC) (HITEC-20170406)},
      pid          = {G:(DE-HGF)POF3-161 / G:(DE-HGF)HGF-YIG-Energy /
                      G:(DE-Juel1)HITEC-20170406},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000351435100010},
      doi          = {10.1002/ejic.201403098},
      url          = {https://juser.fz-juelich.de/record/255767},
}