Gast ::
| Hauptseite > Workflowsammlungen > Öffentliche Einträge > Multijunction Si photocathodes with tunable photovoltages from 2.0 V to 2.8 V for light induced water splitting > print |
| Hauptseite > Workflowsammlungen > Öffentliche Einträge > Multijunction Si photocathodes with tunable photovoltages from 2.0 V to 2.8 V for light induced water splitting > print |
| 001 | 280644 | ||
| 005 | 20240712084454.0 | ||
| 024 | 7 | _ | |a 10.1039/C5EE02393A |2 doi |
| 024 | 7 | _ | |a 1754-5692 |2 ISSN |
| 024 | 7 | _ | |a 1754-5706 |2 ISSN |
| 024 | 7 | _ | |a 2128/9690 |2 Handle |
| 024 | 7 | _ | |a WOS:000367622700017 |2 WOS |
| 024 | 7 | _ | |a altmetric:4681256 |2 altmetric |
| 037 | _ | _ | |a FZJ-2016-00409 |
| 041 | _ | _ | |a English |
| 082 | _ | _ | |a 690 |
| 100 | 1 | _ | |a Urbain, Felix |0 P:(DE-Juel1)156469 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Multijunction Si photocathodes with tunable photovoltages from 2.0 V to 2.8 V for light induced water splitting |
| 260 | _ | _ | |a Cambridge |c 2016 |b RSC Publ. |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1452785011_21607 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 336 | 7 | _ | |a JOURNAL_ARTICLE |2 ORCID |
| 336 | 7 | _ | |a article |2 DRIVER |
| 520 | _ | _ | |a We report on the development of high performance triple and quadruple junction solar cells made of amorphous (a-Si:H) and microcrystalline silicon (μc-Si:H) for the application as photocathodes in integrated photovoltaic–electrosynthetic devices for solar water splitting. We show that the electronic properties of the individual sub cells can be adjusted such that the photovoltages of multijunction devices cover a wide range of photovoltages from 2.0 V up to 2.8 V with photovoltaic efficiencies of 13.6% for triple and 13.2% for quadruple cells. The ability to provide self-contained solar water splitting is demonstrated in a PV-biased electrosynthetic (PV-EC) cell. With the developed triple junction photocathode in the a-Si:H/a-Si:H/μc-Si:H configuration we achieved an operation photocurrent density of 7.7 mA cm−2 at 0 V applied bias using a Ag/Pt layer stack as photocathode/electrolyte contact and ruthenium oxide as counter electrode. Assuming a faradaic efficiency of 100%, this corresponds to a solar-to-hydrogen efficiency of 9.5%. The quadruple junction device provides enough excess voltage to substitute precious metal catalyst, such as Pt by more earth-abundant materials, such as Ni without impairing the solar-to-hydrogen efficiency. |
| 536 | _ | _ | |a 121 - Solar cells of the next generation (POF3-121) |0 G:(DE-HGF)POF3-121 |c POF3-121 |f POF III |x 0 |
| 536 | _ | _ | |0 G:(DE-Juel1)HITEC-20170406 |x 1 |c HITEC-20170406 |a HITEC - Helmholtz Interdisciplinary Doctoral Training in Energy and Climate Research (HITEC) (HITEC-20170406) |
| 588 | _ | _ | |a Dataset connected to CrossRef |
| 700 | 1 | _ | |a Smirnov, Vladimir |0 P:(DE-Juel1)130297 |b 1 |u fzj |
| 700 | 1 | _ | |a Becker, Jan Philipp |0 P:(DE-Juel1)142337 |b 2 |u fzj |
| 700 | 1 | _ | |a Lambertz, Andreas |0 P:(DE-Juel1)130263 |b 3 |u fzj |
| 700 | 1 | _ | |a Yang, Florent |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Ziegler, Jürgen |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Kaiser, Bernhard |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Jaegermann, Wolfram |0 P:(DE-HGF)0 |b 7 |
| 700 | 1 | _ | |a Rau, Uwe |0 P:(DE-Juel1)143905 |b 8 |u fzj |
| 700 | 1 | _ | |a Finger, Friedhelm |0 P:(DE-Juel1)130238 |b 9 |u fzj |
| 773 | _ | _ | |a 10.1039/C5EE02393A |g Vol. 9, no. 1, p. 145 - 154 |0 PERI:(DE-600)2439879-2 |n 1 |p 145 - 154 |t Energy & environmental science |v 9 |y 2016 |x 1754-5706 |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/280644/files/c5ee02393a.pdf |
| 856 | 4 | _ | |y OpenAccess |x icon |u https://juser.fz-juelich.de/record/280644/files/c5ee02393a.gif?subformat=icon |
| 856 | 4 | _ | |y OpenAccess |x icon-1440 |u https://juser.fz-juelich.de/record/280644/files/c5ee02393a.jpg?subformat=icon-1440 |
| 856 | 4 | _ | |y OpenAccess |x icon-180 |u https://juser.fz-juelich.de/record/280644/files/c5ee02393a.jpg?subformat=icon-180 |
| 856 | 4 | _ | |y OpenAccess |x icon-640 |u https://juser.fz-juelich.de/record/280644/files/c5ee02393a.jpg?subformat=icon-640 |
| 856 | 4 | _ | |y OpenAccess |x pdfa |u https://juser.fz-juelich.de/record/280644/files/c5ee02393a.pdf?subformat=pdfa |
| 909 | C | O | |o oai:juser.fz-juelich.de:280644 |p openaire |p open_access |p driver |p VDB |p dnbdelivery |
| 910 | 1 | _ | |a Forschungszentrum Jülich GmbH |0 I:(DE-588b)5008462-8 |k FZJ |b 0 |6 P:(DE-Juel1)156469 |
| 910 | 1 | _ | |a Forschungszentrum Jülich GmbH |0 I:(DE-588b)5008462-8 |k FZJ |b 1 |6 P:(DE-Juel1)130297 |
| 910 | 1 | _ | |a Forschungszentrum Jülich GmbH |0 I:(DE-588b)5008462-8 |k FZJ |b 2 |6 P:(DE-Juel1)142337 |
| 910 | 1 | _ | |a Forschungszentrum Jülich GmbH |0 I:(DE-588b)5008462-8 |k FZJ |b 3 |6 P:(DE-Juel1)130263 |
| 910 | 1 | _ | |a Forschungszentrum Jülich GmbH |0 I:(DE-588b)5008462-8 |k FZJ |b 8 |6 P:(DE-Juel1)143905 |
| 910 | 1 | _ | |a Forschungszentrum Jülich GmbH |0 I:(DE-588b)5008462-8 |k FZJ |b 9 |6 P:(DE-Juel1)130238 |
| 913 | 1 | _ | |a DE-HGF |l Erneuerbare Energien |1 G:(DE-HGF)POF3-120 |0 G:(DE-HGF)POF3-121 |2 G:(DE-HGF)POF3-100 |v Solar cells of the next generation |x 0 |4 G:(DE-HGF)POF |3 G:(DE-HGF)POF3 |b Energie |
| 914 | 1 | _ | |y 2016 |
| 915 | _ | _ | |a Creative Commons Attribution CC BY 3.0 |0 LIC:(DE-HGF)CCBY3 |2 HGFVOC |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0200 |2 StatID |b SCOPUS |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)1160 |2 StatID |b Current Contents - Engineering, Computing and Technology |
| 915 | _ | _ | |a IF >= 20 |0 StatID:(DE-HGF)9920 |2 StatID |b ENERG ENVIRON SCI : 2014 |
| 915 | _ | _ | |a JCR |0 StatID:(DE-HGF)0100 |2 StatID |b ENERG ENVIRON SCI : 2014 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)1150 |2 StatID |b Current Contents - Physical, Chemical and Earth Sciences |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0150 |2 StatID |b Web of Science Core Collection |
| 915 | _ | _ | |a WoS |0 StatID:(DE-HGF)0110 |2 StatID |b Science Citation Index |
| 915 | _ | _ | |a WoS |0 StatID:(DE-HGF)0111 |2 StatID |b Science Citation Index Expanded |
| 915 | _ | _ | |a OpenAccess |0 StatID:(DE-HGF)0510 |2 StatID |
| 915 | _ | _ | |a Allianz-Lizenz / DFG |0 StatID:(DE-HGF)0400 |2 StatID |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)1060 |2 StatID |b Current Contents - Agriculture, Biology and Environmental Sciences |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0310 |2 StatID |b NCBI Molecular Biology Database |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0300 |2 StatID |b Medline |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0199 |2 StatID |b Thomson Reuters Master Journal List |
| 920 | 1 | _ | |0 I:(DE-Juel1)IEK-5-20101013 |k IEK-5 |l Photovoltaik |x 0 |
| 980 | 1 | _ | |a UNRESTRICTED |
| 980 | 1 | _ | |a FullTexts |
| 980 | _ | _ | |a journal |
| 980 | _ | _ | |a VDB |
| 980 | _ | _ | |a UNRESTRICTED |
| 980 | _ | _ | |a I:(DE-Juel1)IEK-5-20101013 |
| 981 | _ | _ | |a I:(DE-Juel1)IMD-3-20101013 |
| Library | Collection | CLSMajor | CLSMinor | Language | Author |
|---|