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@ARTICLE{Ledovskikh:282912,
author = {Ledovskikh, A. V. and Danilov, D. L. and Vliex, M. and
Notten, P. H. L.},
title = {{M}odeling and experimental verification of the
thermodynamic properties of hydrogen storage materials},
journal = {International journal of hydrogen energy},
volume = {41},
number = {6},
issn = {0360-3199},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2016-01651},
pages = {3904 - 3918},
year = {2016},
abstract = {A new mathematical model has been developed describing the
thermodynamics of the hydrogen absorption and desorption
process in Metal Hydrides via the gas phase. This model is
based on first principles chemical and statistical
thermodynamics and takes into account structural changes
occurring inside hydrogen storage materials. A general state
equation has been derived considering the chemical
potentials of reacting species and volume expansion, from
which the equilibrium hydrogen pressure dependence on the
absorbed hydrogen content can be calculated. The model is
able to predict the classical Van ’t Hoff equation from
first-principle analytical expressions and gives more
insight into the various hydrogen storage characteristics.
Pressure-Composition Isotherms have been simulated for
various hydride-forming materials. Excellent agreement
between simulation results and experimental data has been
found in all cases.},
cin = {IEK-9},
ddc = {660},
cid = {I:(DE-Juel1)IEK-9-20110218},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000371654800018},
doi = {10.1016/j.ijhydene.2015.11.038},
url = {https://juser.fz-juelich.de/record/282912},
}