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@ARTICLE{Fisseha:4242,
      author       = {Fisseha, R. and Spahn, H. and Wegener, R. and Hohaus, T.
                      and Brasse, G. and Wissel, H. and Tillmann, R. and Wahner,
                      A. and Koppmann, R. and Kiendler-Scharr, A.},
      title        = {{S}table carbon isotope composition of secondary organic
                      aerosol from ß-pinene oxidation},
      journal      = {Journal of Geophysical Research},
      volume       = {114},
      issn         = {0148-0227},
      address      = {Washington, DC},
      publisher    = {Union},
      reportid     = {PreJuSER-4242},
      pages        = {D02304},
      year         = {2009},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {A chamber study was carried out to investigate the stable
                      carbon isotopic composition (delta C-13) of secondary
                      organic aerosol (SOA) formed from ozonolysis of beta-pinene.
                      beta-Pinene (600 ppb) with a known delta C-13 value
                      $(-30.1\%)$ and 500 ppb ozone were injected into the chamber
                      in the absence of light and the resulting SOA was collected
                      on preheated quartz fiber filters. Furthermore, delta C-13
                      values of the gas-phase beta-pinene and one of its oxidation
                      products, nopinone, were measured using a gas chromatograph
                      coupled to an isotope ratio mass spectrometer (GC-IRMS).
                      beta-Pinene was progressively enriched with the heavy carbon
                      isotope due to the kinetic isotope effect (KIE). The KIE of
                      the reaction of beta-pinene with ozone was measured to be
                      1.0026 ((O3)epsilon 2.6 +/- 1.5 parts per thousand). The
                      delta C-13 value of total secondary organic aerosol was very
                      similar to that of its precursor (average = -29.6 +/- 0.2
                      parts per thousand) independent of experiment time.
                      Nopinone, one of the major oxidation products of
                      beta-pinene, was found in both the gas and aerosol phases.
                      The gas-phase nopinone was heavier than the initial
                      beta-pinene by 1.3 parts per thousand but lighter than the
                      corresponding aerosol-phase nopinone. On average, the
                      gas-phase nopinone was lighter by 2.3 parts per thousand
                      than the corresponding aerosol- phase nopinone. The second
                      product found in the SOA was detected as acetone, but it
                      desorbed from the filter at a higher temperature than
                      nopinone, which indicates that it is a pyrolysis product.
                      The acetone showed a much lower delta C-13 $(-36.6\%)$
                      compared to the initial beta-pinene delta C-13.},
      keywords     = {J (WoSType)},
      cin          = {ICG-2 / ICG-4 / JARA-HPC},
      ddc          = {550},
      cid          = {I:(DE-Juel1)VDB791 / I:(DE-Juel1)VDB793 /
                      $I:(DE-82)080012_20140620$},
      pnm          = {Atmosphäre und Klima / Terrestrische Umwelt},
      pid          = {G:(DE-Juel1)FUEK406 / G:(DE-Juel1)FUEK407},
      shelfmark    = {Meteorology $\&$ Atmospheric Sciences},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000262749100003},
      doi          = {10.1029/2008JD011326},
      url          = {https://juser.fz-juelich.de/record/4242},
}